Bio-Based Polyurethane Resins Derived from Tannin: Source, Synthesis, Characterisation, and Application

被引:30
|
作者
Aristri, Manggar Arum [1 ,2 ]
Lubis, Muhammad Adly Rahandi [1 ]
Iswanto, Apri Heri [3 ,4 ]
Fatriasari, Widya [1 ]
Sari, Rita Kartika [2 ]
Antov, Petar [5 ]
Gajtanska, Milada [6 ]
Papadopoulos, Antonios N. [7 ]
Pizzi, Antonio [8 ]
机构
[1] Natl Res & Innovat Agcy, Cibinong Sci Ctr, Res Ctr Biomat, Cibinong 16911, Indonesia
[2] IPB Univ, Fac Forestry & Environm, Dept Forest Prod, Bogor 16680, Indonesia
[3] Univ Sumatera Utara, Dept Forest Prod, Fac Forestry, Medan 20155, Indonesia
[4] Univ Sumatera Utara, JATI Sumatran Forestry Anal Study Ctr, Medan 20155, Indonesia
[5] Univ Forestry, Fac Forest Ind, Sofia 1797, Bulgaria
[6] Tech Univ Zvolen, Fac Wood Sci & Technol, Zvolen 96001, Slovakia
[7] Int Hellen Univ, Dept Forestry & Nat Environm, Lab Wood Chem & Technol, GR-66100 Drama, Greece
[8] Univ Lorraine, LERMAB, F-88000 Epinal, France
来源
FORESTS | 2021年 / 12卷 / 11期
关键词
bio-based polyurethane; extraction; synthesis; tannin; tannin source; C-13 NMR ANALYSIS; HYDROLYZABLE TANNINS; MALDI-TOF; CORROSION INHIBITION; CONDENSED TANNINS; GALLIC ACID; FOAMS; POLYPHENOLS; EXTRACTS; BARK;
D O I
10.3390/f12111516
中图分类号
S7 [林业];
学科分类号
0829 ; 0907 ;
摘要
Tannins are soluble, astringent secondary phenolic metabolites generally obtained from renewable natural resources, and can be found in many plant parts, such as fruits, stems, leaves, seeds, roots, buds, and tree barks, where they have a protective function against bacterial, fungal, and insect attacks. In general, tannins can be extracted using hot water or organic solvents from the bark, leaves, and stems of plants. Industrially, tannins are applied to produce adhesives, wood coatings, and other applications in the wood and polymer industries. In addition, tannins can also be used as a renewable and environmentally friendly material to manufacture bio-based polyurethanes (bio-PUs) to reduce or eliminate the toxicity of isocyanates used in their manufacture. Tannin-based bio-PUs can improve the mechanical and thermal properties of polymers used in the automotive, wood, and construction industries. The various uses of tannins need to be put into perspective with regards to possible further advances and future potential for value-added applications. Tannins are employed in a wide range of industrial applications, including the production of leather and wood adhesives, accounting for almost 90% of the global commercial tannin output. The shortage of natural resources, as well as the growing environmental concerns related to the reduction of harmful emissions of formaldehyde or isocyanates used in the production of polyurethanes, have driven the industrial and academic interest towards the development of tannin-based bio-PUs as sustainable alternative materials with satisfactory characteristics. The aim of the present review is to comprehensively summarize the current state of research in the field of development, characterization, and application of tannin-derived, bio-based polyurethane resins. The successful synthesis process of the tannin-based bio-PUs was characterized by Fourier-transform infrared spectroscopy (FTIR), differential scanning calorimetry (DSC), thermogravimetric analysis (TGA), MALDI-TOF mass spectrometry, and gel permeation chromatography (GPC) analyses.
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页数:23
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