Ammonia was synthesized from its elements at atmospheric pressure in a solid state proton (H+)-conducting cell-reactor. Hydrogen was flowing over the anode and was converted into protons that were transported through the solid electrolyte and reached the cathode (palladium) over which nitrogen was passing. At 570 degrees C and atmospheric pressure, greater than 78 percent of the electrochemically supplied hydrogen was converted into ammonia. The thermodynamic requirement for a high-pressure process is eliminated.
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Kyoto Univ, Dept Fundamental Energy Sci, Grad Sch Energy Sci, Kyoto 6068501, JapanKyoto Univ, Dept Fundamental Energy Sci, Grad Sch Energy Sci, Kyoto 6068501, Japan
Murakami, T
Nohira, T
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机构:Kyoto Univ, Dept Fundamental Energy Sci, Grad Sch Energy Sci, Kyoto 6068501, Japan
Nohira, T
Ogata, YH
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机构:Kyoto Univ, Dept Fundamental Energy Sci, Grad Sch Energy Sci, Kyoto 6068501, Japan
Ogata, YH
Ito, Y
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机构:Kyoto Univ, Dept Fundamental Energy Sci, Grad Sch Energy Sci, Kyoto 6068501, Japan
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Key Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
School of Physics, Dalian University of TechnologyKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
李瑶
陈兆权
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Anhui Province Key Laboratory of Power Electronics and Electrical Control, Anhui University ofKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
陈兆权
李思思
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Key Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
School of Physics, Dalian University of TechnologyKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
李思思
冯旖
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Key Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
School of Physics, Dalian University of TechnologyKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
冯旖
郑直
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Key Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
School of Physics, Dalian University of TechnologyKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
郑直
杨徳正
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Key Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education
School of Physics, Dalian University of TechnologyKey Laboratory of Materials Modification by Laser, Ion, and Electron Beams (Dalian University of Technology), Ministry of Education