A high-performance, durable and low-cost proton exchange membrane electrolyser with stainless steel components

被引:95
|
作者
Stiber, S. [1 ]
Sata, N. [1 ]
Morawietz, T. [1 ]
Ansar, S. A. [1 ]
Jahnke, T. [2 ]
Lee, J. K. [3 ]
Bazylak, A. [3 ]
Fallisch, A. [4 ]
Gago, A. S. [1 ]
Friedrich, K. A. [1 ,5 ]
机构
[1] German Aerosp Ctr DLR, Inst Engn Thermodynam Electrochem Energy Technol, Pfaffenwaldring 38-40, D-70569 Stuttgart, Germany
[2] German Aerosp Ctr DLR, Inst Engn Thermodynam Computat Electrochem, Pfaffenwaldring 38-40, D-70569 Stuttgart, Germany
[3] Univ Toronto, Inst Sustainable Energy, Fac Appl Sci & Engn, Dept Mech & Ind Engn, Toronto, ON M5S 3G8, Canada
[4] Fraunhofer Inst Solare Energiesyst ISE, Heidenhofstr 2, D-79110 Freiburg, Germany
[5] Univ Stuttgart, Inst Bldg Energet Thermal Engn & Energy Storage I, Pfaffenwaldring 31, D-70569 Stuttgart, Germany
基金
欧盟地平线“2020”;
关键词
POROUS TRANSPORT LAYER; WATER ELECTROLYSIS; BIPOLAR PLATES; DIFFUSION LAYERS; CATALYST; CELLS; GAS; DEGRADATION; TITANIUM;
D O I
10.1039/d1ee02112e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Proton exchange membrane water electrolysis (PEMWE) is the most promising technology for sustainable hydrogen production. However, it has been too expensive to compete with current state-of-the-art technologies due to the high cost of titanium bipolar plates (BPPs) and porous transport layers (PTLs). Here, we report a high-performance, durable and low-cost PEMWE cell with coated stainless steel (ss) BPPs and PTLs. When using uncoated ss components in the PEMWE cell, the cell depolarizes rapidly, reaching 2 V at only 0.15 A cm(-2). After the application of non-precious metal coatings of Ti and Nb/Ti on the ss-BPP and ss-PTL, respectively, the current density can be increased by a factor of 13 while maintaining the same performance. Extensive physical and electrochemical characterization supported by pore network modelling shows that the Nb/Ti coating on the ss-PTL leads to efficient water and gas transport at the interface with the anode. The PEMWE cell with coated ss components was evaluated in an accelerated stress test (AST) for more than 1000 h. No sign of Fe contamination in either the membrane or the electrodes is observed at the end of the test. With our results, we demonstrate that PEMWE cells can be manufactured almost entirely in ss, facilitating an unprecedented cost reduction in this technology and advancing the widespread use of green H-2.
引用
收藏
页码:109 / 122
页数:15
相关论文
共 50 条
  • [41] Low-cost and high-performance selenium indoor photovoltaics
    Wei, Zhouqing
    Lu, Wenbo
    Li, Zongbao
    Feng, Mingjie
    Yan, Bin
    Hu, Jin-Song
    Xue, Ding-Jiang
    JOURNAL OF MATERIALS CHEMISTRY A, 2023, 11 (44) : 23837 - 23843
  • [42] LOW-COST AUDIO VCA HAS HIGH-PERFORMANCE
    SIMS, M
    EDN, 1995, 40 (02) : 95 - 95
  • [43] Activation of low-cost stainless-steel electrodes for efficient and stable anion-exchange membrane water electrolysis
    Jiang, Tao
    Zouridi, Leila
    Li, Nannan
    Binas, Vassilios
    Stuart, Marc. C. A.
    Aravind, P.V.
    Jayawardhana, Bayu
    Pescarmona, Paolo P.
    Kyriakou, Vasileios
    Journal of Materials Chemistry A, 2024, 12 (43) : 29909 - 29922
  • [44] Design of compact RF components for low-cost high-performance wireless front-ends
    Zheng, G
    Pinel, S
    Lim, K
    Li, R
    Tentzeris, M
    Papapolymerou, J
    Laskar, J
    Lenoir, B
    Blondy, P
    Baillargeat, D
    Guillon, P
    2002 3RD INTERNATIONAL CONFERENCE ON MICROWAVE AND MILLIMETER WAVE TECHNOLOGY PROCEEDINGS, 2002, : 259 - 262
  • [45] Polypyrrole/sargassum activated carbon modified stainless-steel sponge as high-performance and low-cost bioanode for microbial fuel cells
    Wu, Gaoming
    Bao, Han
    Xia, Zheng
    Yang, Bin
    Lei, Lecheng
    Li, Zhongjian
    Liu, Chunxian
    JOURNAL OF POWER SOURCES, 2018, 384 : 86 - 92
  • [46] Low-cost, high performance optoelectronic components for antenna remoting
    Prince, JL
    Roussell, HV
    Ackerman, EI
    Knowlton, R
    Cox, CH
    OPTICAL AND QUANTUM ELECTRONICS, 1998, 30 (11-12) : 1051 - 1063
  • [47] Low-cost, high performance optoelectronic components for antenna remoting
    J. L. Prince
    H. V. Roussell
    E. I. Ackerman
    R. Knowlton
    C. H. Cox III
    Optical and Quantum Electronics, 1998, 30 : 1051 - 1063
  • [48] Enhanced performance of Ti–Nb–N film modified 316L stainless steel and Ti bipolar plates for proton exchange membrane water electrolyser
    Yu, Zhongxiu
    Luo, Xiejing
    Chang, Luqi
    Ding, Yingyu
    Yao, Jizheng
    Deng, Zhanfeng
    Dong, Chaofang
    Journal of Materials Research and Technology, 2024, 33 : 2478 - 2488
  • [49] Acid-durable, high-performance cobalt phosphide catalysts for hydrogen evolution in proton exchange membrane water electrolysis
    Yoon, Young
    Kim, Hoyoung
    Kim, Soo-Kil
    Kim, Jae Jeong
    INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2021, 45 (11) : 16842 - 16855
  • [50] Cost Analysis for Durable Proton Exchange Membrane in PEM Fuel Cells
    Taleb, Ali
    Kjeang, Erik
    Maine, Elicia
    PICMET '12: PROCEEDINGS - TECHNOLOGY MANAGEMENT FOR EMERGING TECHNOLOGIES, 2012, : 2943 - 2950