Electron Ionization of Size-Selected Positively and Negatively Charged Helium Droplets

被引：4
|
作者：
Laimer, Felix [1 ]
Zappa, Fabio [1 ]
Gruber, Elisabeth [1 ]
Scheier, Paul [1 ]
机构：
[1] Univ Innsbruck, Inst Ionenphys & Angew Phys, Tech Str 25, A-6020 Innsbruck, Austria
来源：
ATOMS | 2021年 / 9卷 / 04期
基金：
奥地利科学基金会;
关键词：
electron ionization; electron capture; helium droplets; cross section; IMPACT IONIZATION; CROSS-SECTIONS; INFRARED-SPECTROSCOPY; IONS; FRAGMENTATION; COLLISIONS; MOLECULES; CLUSTERS; CAPTURE; ATOMS;
D O I：
10.3390/atoms9040074
中图分类号：
O64 [物理化学（理论化学）、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号：
070203 ; 070304 ; 081704 ; 1406 ;
摘要：
A beam of size-selected charged helium droplets was crossed with an electron beam, and the ion efficiency curves for the product droplets in all different charge states were recorded. We estimate that the selected helium droplets on their passage through the electron beam are hit by several hundred electrons which can interact with the individual He atoms of the droplets. Reaction channels corresponding to the removal or capture of up to eight electrons were identified, and in all cases, inelastic scattering and the formation of metastable helium played a significant role.
引用
收藏
页数：15
相关论文
共 50 条
  • [41] Electron-impact multiple-ionization of negatively-charged fullerene ions
    Hathiramani, D
    Aichele, K
    Arnold, W
    Huber, K
    Salzborn, E
    Scheier, P
    MOLECULAR MATERIALS, 2000, 13 (1-4): : 343 - 348
  • [42] SIZE DISTRIBUTIONS OF NEGATIVELY AND POSITIVELY CHARGED CLUSTERS - CO2 AND N2O
    KNAPP, M
    KREISLE, D
    ECHT, O
    SATTLER, K
    RECKNAGEL, E
    SURFACE SCIENCE, 1985, 156 (JUN) : 313 - 320
  • [43] Plasmonic evolution of atomically size-selected Au clusters by electron energy loss spectrum
    Lu, Siqi
    Xie, Lin
    Lai, Kang
    Chen, Runkun
    Cao, Lu
    Hu, Kuojuei
    Wang, Xuefeng
    Han, Jinsen
    Wan, Xiangang
    Wan, Jianguo
    Dai, Qing
    Song, Fengqi
    He, Jiaqing
    Dai, Jiayu
    Chen, Jianing
    Wang, Zhenlin
    Wang, Guanghou
    NATIONAL SCIENCE REVIEW, 2021, 8 (12)
  • [44] Strong field induced ion and electron emission from size-selected metal clusters
    Raspe, K.
    Kazak, L.
    Iwe, N.
    Krebs, B.
    Martinez, F.
    Meiwes-Broer, K. -h.
    Tiggesbaeumker, J.
    PHYSICAL REVIEW RESEARCH, 2024, 6 (04):
  • [45] Plasmonic evolution of atomically size-selected Au clusters by electron energy loss spectrum
    Siqi Lu
    Lin Xie
    Kang Lai
    Runkun Chen
    Lu Cao
    Kuojuei Hu
    Xuefeng Wang
    Jinsen Han
    Xiangang Wan
    Jianguo Wan
    Qing Dai
    Fengqi Song
    Jiaqing He
    Jiayu Dai
    Jianing Chen
    Zhenlin Wang
    Guanghou Wang
    National Science Review, 2021, 8 (12) : 20 - 28
  • [46] Fine structure of negatively and positively charged excitons in semiconductor quantum dots: Electron-hole asymmetry
    Ediger, M.
    Bester, G.
    Gerardot, B. D.
    Badolato, A.
    Petroff, P. M.
    Karrai, K.
    Zunger, A.
    Warburton, R. J.
    PHYSICAL REVIEW LETTERS, 2007, 98 (03)
  • [47] Incorporating Electro-Epoxidation into Electrospray Ionization Mass Spectrometry for Simultaneous Analysis of Negatively and Positively Charged Unsaturated Glycerophospholipids
    Tang, Shuli
    Fan, Licheng
    Cheng, Heyong
    Yan, Xin
    JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY, 2021, 32 (09) : 2288 - 2295
  • [48] Electron impact ionization studies with the amino acid valine in the gas phase and (hydrated) in helium droplets
    S. Denifl
    I. Mähr
    F. Ferreira da Silva
    F. Zappa
    T. D. Märk
    P. Scheier
    The European Physical Journal D, 2009, 51 : 73 - 79
  • [49] Electron impact ionization studies with the amino acid valine in the gas phase and (hydrated) in helium droplets
    Denifl, S.
    Maehr, I.
    da Silva, F. Ferreira
    Zappa, F.
    Mark, T. D.
    Scheier, P.
    EUROPEAN PHYSICAL JOURNAL D, 2009, 51 (01): : 73 - 79
  • [50] Size-selected (2-10 nm) gold nanoparticles for matrix assisted laser desorption ionization of peptides
    McLean, John A.
    Stumpo, Katherine A.
    Russel, David H.
    1600, American Chemical Society, Columbus, United States (127):
12345