Facile synthesis of Y-doped graphitic carbon nitride with enhanced photocatalytic performance

被引:56
|
作者
Wang, Yangang [1 ]
Li, Yaguang [1 ]
Bai, Xia [1 ]
Cai, Qing [1 ]
Liu, Chenglu [1 ]
Zuo, Yuanhui [1 ]
Kang, Shifei [1 ]
Cui, Lifeng [1 ]
机构
[1] Univ Shanghai Sci & Technol, Dept Environm Sci & Engn, Shanghai 200093, Peoples R China
基金
中国国家自然科学基金;
关键词
Graphitic carbon nitride; Y doping; Visible-light-driven photocatalyst; Photocatalytic degradation; VISIBLE-LIGHT IRRADIATION; OXYGEN REDUCTION; PHENOL; G-C3N4; OXIDATION; CATALYSTS; DEGRADATION; POLYMERS; BENZENE; TIO2;
D O I
10.1016/j.catcom.2016.06.020
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Yttrium-doped graphitic carbon nitride (Y/g-C3N4) catalysts were prepared via a facile pyrolysis method with urea used as a precursor and yttrium nitrate as the Y source. Characterization results show that an appropriate doping ratio of Y can be embedded into in-planes of g-C3N4. The Y/g-C3N4 catalysts are characterized by hierarchical porosity, large specific surface area, and large pore volume. Introduction of Y species effectively extends the spectral response of g-C3N4 from ultraviolet to visible region and decelerates the recombination of photogenerated electrons and holes. Because of these properties, the Y/g-C3N4 catalysts show an enhanced photocatalytic performance in rhodamine B degradation under visible light. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:179 / 182
页数:4
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