Stable Hematite Nanosheet Photoanodes for Enhanced Photoelectrochemical Water Splitting

被引:279
|
作者
Peerakiatkhajohn, Piangjai [1 ,2 ]
Yun, Jung-Ho [1 ,2 ]
Chen, Hongjun [1 ,2 ]
Lyu, Miaoqiang [1 ,2 ]
Butburee, Teera [1 ,2 ]
Wang, Lianzhou [1 ,2 ]
机构
[1] Univ Queensland, Sch Chem Engn, Nanomat Ctr, St Lucia, Qld 4072, Australia
[2] Univ Queensland, AIBN, St Lucia, Qld 4072, Australia
基金
澳大利亚研究理事会;
关键词
ALPHA-FE2O3 NANOTUBE ARRAYS; THIN-FILMS; SILVER NANOPARTICLES; CO-PI; SOLAR; OXIDATION; GROWTH; ELECTRODEPOSITION; PHOTOOXIDATION; SEMICONDUCTORS;
D O I
10.1002/adma.201601525
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A vertically grown hematite nanosheet film modified with Ag nanoparticles (NPs) and Co-Pi cocatalyst exhibits a remarkably high photocurrent density of 4.68 mA cm(-2) at 1.23 V versus RHE. The Ag NPs leads to significantly improved light harvesting and better charge transfer, while the Co-Pi facilitates a highly stable oxygen evolution process. This photoelectrode design provides more efficient photoelectrochemical systems for solar-energy conversion.
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页码:6405 / +
页数:7
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