Multi-scale pore morphologies of a compressed gas diffusion layer for polymer electrolyte fuel cells

被引:27
|
作者
Yoshimune, Wataru [1 ]
Kato, Satoru [1 ]
Yamaguchi, Satoshi [1 ]
机构
[1] Toyota Cent Res & Dev Labs Inc, 41-1 Yokomichi, Nagakute, Aichi 4801192, Japan
关键词
Polymer electrolyte fuel cell; Gas diffusion layer; Micro-porous layer; Compression; Mercury intrusion porosimetry; X-ray computed micro-tomography; MICRO-POROUS LAYERS; RAY COMPUTED-TOMOGRAPHY; THERMAL-CONDUCTIVITY; OXYGEN-TRANSPORT; WATER; MECHANISMS; RESISTANCE; STRESS; MEDIA; GDL;
D O I
10.1016/j.ijheatmasstransfer.2020.119537
中图分类号
O414.1 [热力学];
学科分类号
摘要
Understanding the pore morphologies of a compressed gas diffusion layer is critical to improve the performance of polymer electrolyte fuel cells. In this study, the effect of compression on the cell performance was investigated. Increasing the gas diffusion layer compression increases oxygen transport resistance. Moreover, the pore morphologies of the compressed gas diffusion layer were investigated using mercury intrusion porosimetry with a simple compression device and synchrotron X-ray computed microtomography. The average pore diameter of the fibrous substrate reduced applying compression pressure, whereas that of the micro-porous layer remained unchanged even at high compression (38.6%). In addition, the oxygen transport resistance calculated from the structural parameters of a compressed gas diffusion layer, where porosity and pore diameter are explanatory factors, was in good agreement with the oxygen transport resistance obtained by fuel cell testing. (C) 2020 Elsevier Ltd. All rights reserved.
引用
收藏
页数:5
相关论文
共 50 条
  • [11] Development of carbon-filled gas diffusion layer for polymer electrolyte fuel cells
    Han, M.
    Chan, S. H.
    Jiang, S. P.
    JOURNAL OF POWER SOURCES, 2006, 159 (02) : 1005 - 1014
  • [12] Investigation of convective transport in the gas diffusion layer used in polymer electrolyte fuel cells
    Beruski, Otavio
    Lopes, Thiago
    Kucernak, Anthony R. J.
    Perez, Joelma
    PHYSICAL REVIEW FLUIDS, 2017, 2 (10):
  • [13] The Effect of Clamping Pressure on Gas Diffusion Layer Performance in Polymer Electrolyte Fuel Cells
    El-kharouf, A.
    Steinberger-Wilckens, R.
    FUEL CELLS, 2015, 15 (06) : 802 - 812
  • [14] Polymer Electrolyte Fuel Cells Lifetime Prediction by a Full Multi-Scale Modeling Approach
    Gerard, M.
    Robin, C.
    Chandesris, M.
    Schott, P.
    POLYMER ELECTROLYTE FUEL CELLS 16 (PEFC 16), 2016, 75 (14): : 35 - 43
  • [15] Does the thermal conductivity of gas diffusion layer matter in polymer electrolyte fuel cells?
    Csoklich, Christoph
    Sabharwal, Mayank
    Schmidt, Thomas J.
    Buchi, Felix N.
    JOURNAL OF POWER SOURCES, 2022, 540
  • [16] The Role of Gas Diffusion Layer in Cationic Contamination and Mitigation in Polymer Electrolyte Fuel Cells
    Uddin, Md. Aman
    Park, Jaehyung
    Wang, Xiaofeng
    Qi, Jing
    Pasaogullari, Ugur
    Bonville, Leonard
    Molter, Trent
    POLYMER ELECTROLYTE FUEL CELLS 14, 2014, 64 (03): : 537 - 544
  • [17] Effects of the cathode gas diffusion layer characteristics on the performance of polymer electrolyte fuel cells
    Antolini, E
    Passos, RR
    Ticianelli, EA
    JOURNAL OF APPLIED ELECTROCHEMISTRY, 2002, 32 (04) : 383 - 388
  • [18] New Porous Carbon Materials as Gas Diffusion Layer for Polymer Electrolyte Fuel Cells
    Okada, Tatsuhiro
    Kyotani, Mutsumasa
    Yamamoto, Tomoaki
    Terada, Naofumi
    Yoshida, Shin-ichi
    ELECTROCHEMISTRY, 2020, 88 (05) : 423 - 428
  • [19] Effects of the cathode gas diffusion layer characteristics on the performance of polymer electrolyte fuel cells
    E. Antolini
    R.R. Passos
    E.A. Ticianelli
    Journal of Applied Electrochemistry, 2002, 32 : 383 - 388
  • [20] Determination of oxygen transport resistance in gas diffusion layer for polymer electrolyte fuel cells
    Wan, Z. H.
    Zhong, Q.
    Liu, S. F.
    Jin, A. P.
    Chen, Y. N.
    Tan, J. T.
    Pan, M.
    INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2018, 42 (06) : 2225 - 2233