Atomic-scale dissipation processes in dynamic force spectroscopy

被引:36
|
作者
Kawai, Shigeki [1 ]
Canova, Filippo Federici [2 ,3 ]
Glatzel, Thilo [1 ]
Foster, Adam S. [2 ,3 ]
Meyer, Ernst [1 ]
机构
[1] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland
[2] Tampere Univ Technol, Dept Phys, FI-33010 Tampere, Finland
[3] Aalto Univ, Dept Appl Phys, FI-00076 Aalto, Finland
基金
瑞士国家科学基金会;
关键词
FREQUENCY; MICROSCOPE; OPERATION; ADHESION; ENERGY; MODE;
D O I
10.1103/PhysRevB.84.115415
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A systematic distance-dependent measurement of the quasistatic tip-sample interactions reveals a hidden stochastic dissipative interaction of the atomic-scale contact in dynamic force microscopy. By comparison of experiment with detailed molecular dynamics simulations, we demonstrate that the infrequently observed hysteresis loops are attributed to the formation of atomic chains during tip retraction. These lead to a large magnitude of energy dissipation in a single cycle and dominate the average measured dissipation, while also leading to differences in the forces measured in static and dynamic force microscopy. This paper provides quantitative force measurements and insights into atomic-scale dissipation processes.
引用
收藏
页数:9
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