Host-Guest chemistry based on solid-state pillar[n]arenes

被引：78

作者：

Ohtani, Shunsuke ^{[1
]}

Kato, Kenichi ^{[1
]}

Fa, Shixin ^{[1
]}

Ogoshi, Tomoki ^{[1
,2
]}

机构：

[1] Kyoto Univ, Grad Sch Engn, Dept Synthet Chem & Biol Chem, Nishikyo Ku, Kyoto 6158510, Japan

[2] Kanazawa Univ, WPI Nano Life Sci Inst WPI NanoLSI, Kakuma Machi, Kanazawa, Ishikawa 9201192, Japan

来源：

COORDINATION CHEMISTRY REVIEWS | 2022年 / 462卷

关键词：

Pillar[n]arene; Host-guest chemistry; Solid-state complexation; Supramolecular chemistry; NONPOROUS ADAPTIVE CRYSTALS; HIGH-YIELD SYNTHESIS; MOLECULAR RECOGNITION; SELECTIVE COMPLEXATION; SUPRAMOLECULAR POLYMERS; CUCURBITURIL HOMOLOGS; ORGANIC FRAMEWORKS; INCLUSION COMPLEX; THIN-FILMS; SEPARATION;

D O I：

10.1016/j.ccr.2022.214503

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

Pillar[n]arenes, which were first reported by our group in 2008, are a new type of pillar-shaped host molecule in host-guest chemistry with versatile and unique host-guest behaviors. Host-guest complexation is mostly investigated in solution systems, where both the host and guest molecules are normally dissolved in solvent. Compared with normal host-guest complexation in solvents, solid-state host-guest complexation can offer the following advantages and characteristics: (i) Cavity-size dependent host- guest complexation, (ii) efficient host-guest complexation, and (iii) easy host-guest complex isolation and solid-state pillar[n]arene reuse. In this review, we discuss the recent development of solid-state host-guest complexation using crystalline pillar[n]arenes, two or three-dimensional networks containing pillar[n]arenes, including hydrogen-bonded organic frameworks (HOFs), and metal-organic frameworks (MOFs), pillar[n]arene-assembled surfaces, and solid-state organic polymers containing pillar[n]arenes. (C)& nbsp;2022 Elsevier B.V. All rights reserved.

引用

页数：34

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