Classical Wigner phase space approximation to cumulative matrix elements in coherent control

被引：9

作者：

McQuarrie, BR

Abrashkevich, DG

Brumer, P ^{[1
]}

机构：

[1] Univ Minnesota Morris, Div Sci & Math, Morris, MN 56267 USA

[2] Univ Toronto, Dept Chem, Chem Phys Theory Grp, Toronto, ON M5S 3H6, Canada

来源：

JOURNAL OF CHEMICAL PHYSICS | 2003年 / 119卷 / 07期

关键词：

D O I：

10.1063/1.1590962

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The classical limit of the Wigner-Weyl representation is used to approximate products of bound-continuum matrix elements that are fundamental to many coherent control computations. The range of utility of the method is quantified through an examination of model problems, single-channel Na-2 dissociation and multiarrangement channel photodissociation of CH2IBr. Very good agreement with the exact quantum results is found for a wide range of system parameters. (C) 2003 American Institute of Physics.

引用

页码：3606 / 3618

页数：13

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