Linear and nonlinear optical characteristics of all-inorganic perovskite CsPbBr3 quantum dots modified by hydrophobic zeolites

被引:41
|
作者
Li, Ruxue [1 ,2 ]
Wei, Zhipeng [1 ]
Zhao, Haixia [1 ]
Yu, Hongrui [1 ]
Fang, Xuan [1 ]
Fang, Dan [1 ]
Li, Junzi [3 ]
He, Tingchao [3 ]
Chen, Rui [2 ]
Wang, Xiaohua [1 ]
机构
[1] Changchun Univ Sci & Technol, Sch Sci, State Key Lab High Power Semicond Lasers, 7089 Wei Xing Rd, Changchun 130022, Jilin, Peoples R China
[2] South Univ Sci & Technol China, Dept Elect & Elect Engn, Shenzhen 518055, Guangdong, Peoples R China
[3] Shenzhen Univ, Coll Phys & Energy, Shenzhen 518060, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
STIMULATED-EMISSION; 2-PHOTON ABSORPTION; HALIDE PEROVSKITES; ENHANCED STABILITY; HIGH-EFFICIENCY; NANOCRYSTALS; NANOCOMPOSITES; SATURATION; CSPBX3; AIR;
D O I
10.1039/c8nr07256f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
All-inorganic perovskite quantum dots (QDs) have been considered as outstanding candidates for high-performance optoelectronic device applications. However, the chemical and optical stabilities restrict their device applications. In this paper, hydrophobic zeolites were proposed to modify CsPbBr3 QDs to prevent water influence while achieving good dispersion. These hybrid luminescent materials possess high internal quantum efficiency (IQE, similar to 81%@3.52 W cm(-2)) and low dissociation levels that give rise to improved optical stability in terms of temperature and time. More interesting, it is found that this nanocomposite is able to maintain its optical limiting performance under intensive laser illumination. This paper discusses the linear and nonlinear optical characteristics of CsPbBr3 QDs, which would be of great importance for both fundamental physics investigation and practical multiphoton applications.
引用
收藏
页码:22766 / 22774
页数:9
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