Cascaded Membrane Processes for Post-Combustion CO2 Capture

被引：27

作者：

Zhao, Li ^{[1
]}

Riensche, Ernst ^{[1
]}

Weber, Michael ^{[1
]}

Stolten, Detlef ^{[1
]}

机构：

[1] Forschungszentrum Julich, Inst Energy & Climate Res Fuel Cells, D-52425 Julich, Germany

来源：

CHEMICAL ENGINEERING & TECHNOLOGY | 2012年 / 35卷 / 03期

关键词：

Cascaded membrane process; CO2; N2; membrane; Dewatering; Post-combustion; Pressure loss; CARBON-DIOXIDE; FLUE-GAS; TECHNOLOGIES;

D O I：

10.1002/ceat.201100462

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

CO2 fugacity difference is the driving force for CO2-selective membranes used in post-combustion capture. The ambient pressure of the flue gas makes it very difficult to use only a single membrane stage to achieve the CO2 purity required by pipeline transport and storage, e.g., 95?mol.-%. On the basis of a general multi-stage membrane concept, an energy-efficient membrane cascade is developed. The correlation of energy consumption and membrane area of a cascaded membrane process is investigated, considering 50?%, 70?%, and 90?% degree of CO2 separation. In addition to an idealized flue gas consisting of N2 and CO2 only, also a quasi-real flue gas is studied. Pressure loss in membrane modules and their influence on process energy consumption are discussed.

引用

页码：489 / 496

页数：8

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