Petroleum coke;
low-rank coal;
coal water slurries;
rheological behavior;
slurryability;
gasification;
GASIFICATION REACTIVITY;
WATER SLURRY;
PERFORMANCE;
STABILITY;
PETCOKE;
LIGNITE;
D O I:
10.1080/19392699.2021.1954915
中图分类号:
TE [石油、天然气工业];
TK [能源与动力工程];
学科分类号:
0807 ;
0820 ;
摘要:
Gasification is an efficient and environmentally friendly treatment process for petroleum coke. But the rheology and stability of petroleum coke-water slurries (PWS) do not meet the feeding requirements of gasification. This study blends Hami coal (HM) with two petroleum cokes (Lianyungang (LYG) and Lanqiao (LQ)) to prepare high quality slurries. The results indicate that the properties of petroleum coke have significant effects on the blending slurries. With a certain amount of oxygen-containing functional groups and small molecular branched chains, LYG could be blended with HM to prepare high quality slurries with a maximum solid loading of 64.87%, static stability of 4 days, and a shear-thinning rheological behavior. However, HM could not provide the same benefits to the slurries prepared with LQ, as LQ exhibits a higher degree of aromatic carbonization. Aggregation state of the particles is the main reason behind this difference.
机构:
Hokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, Japan
Mochizuki, Yuuki
Kubota, Yukihiro
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机构:
Nippon Steel & Sumitomo Met Corp, Tech Res & Dev Bur, Chiba 2938511, JapanHokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, Japan
Kubota, Yukihiro
Uebo, Kazuya
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机构:
Nippon Steel & Sumitomo Met Corp, Tech Res & Dev Bur, Chiba 2938511, JapanHokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, Japan
Uebo, Kazuya
Tsubouchi, Naoto
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h-index: 0
机构:
Hokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Ctr Adv Res Energy & Mat, Kita Ku, Kita 13 Nishi 5, Sapporo, Hokkaido 0608628, Japan