Recovery of uranium (VI) from aqueous solutions by the polyethyleneimine-functionalized reduced graphene oxide/molybdenum disulfide composition aerogels

被引:30
|
作者
Guo, Dongxuan [1 ]
Song, Xiumei [3 ]
Zhang, Lulu [1 ]
Chen, Weiwen [1 ]
Chu, Daiwei [1 ]
Tan, Lichao [1 ,2 ]
机构
[1] Harbin Univ Sci & Technol, Coll Chem & Environm Engn, Sch Mat Sci & Engn, Harbin 150040, Peoples R China
[2] Harbin Engn Univ, Minist Educ, Key Lab Superlight Mat & Surface Technol, Harbin 150001, Peoples R China
[3] Harbin Inst Technol, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China
基金
中国博士后科学基金;
关键词
Uranium (VI); Adsorption; Polyethyleneimine; MoS2; Composition aerogels; METHYLENE-BLUE; ADSORPTION; SEAWATER; REMOVAL; EXTRACTION; NANOSHEETS; STRATEGY; GELATION; MWCNT; TIO2;
D O I
10.1016/j.jtice.2019.09.029
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
In this work, we have developed a facile route for the fabrication of polyethyleneimine-functionalized reduced graphene oxide/molybdenum disulfide composition aerogels (PEI-rGO/MoS2 CAs). The as-obtained nanomaterial (PEI-rGO/MoS2 CAs) is characterized by using scanning electron microscopy, transmission electron microscopy, Fourier-transform infrared spectroscopy, X-ray diffraction and X-ray photoelectron spectroscopy measurements. The different parameters regulating the adsorption of uranium (VI) such as contact time, pH and temperature are texted. The results show that the adsorption processes of uranium (VI) onto PEI-rGO/MoS2 CAs-3 are spontaneous and endothermic and well follow pseudo-second-order and Langmuir isotherm model. The equilibrium time and maximum adsorption capacity of PEI-rGO/MoS2 CAs-3 are 350 min and 184.53 mg g(-1). Therefore, PEI-rGO/MoS2 CAs holds the potential as promising adsorbent for the adsorption of uranium (VI). (C) 2019 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:198 / 205
页数:8
相关论文
共 50 条
  • [21] Sorption of uranium from aqueous solutions with graphene oxide
    Wang, Chun Li
    Li, Yan
    Liu, Chun Li
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2015, 304 (03) : 1017 - 1025
  • [22] Graphene Oxide-Cellulose Composite for the Adsorption of Uranium(VI) from Dilute Aqueous Solutions
    Yang, Aili
    Wu, Junhong
    Huang, C. P.
    JOURNAL OF HAZARDOUS TOXIC AND RADIOACTIVE WASTE, 2018, 22 (02)
  • [23] Fabrication of porous polyethyleneimine-functionalized chitosan/Span 80 microspheres for adsorption of diclofenac sodium from aqueous solutions
    Jiang, Fangyuan
    Zhang, Dachao
    Ouyang, Xiao-kun
    Yang, Li-Ye
    SUSTAINABLE CHEMISTRY AND PHARMACY, 2021, 21
  • [24] Recovery of uranium(VI) from aqueous solution by amidoxime functionalized wool fibers
    Zhonglong Yin
    Jie Xiong
    Min Chen
    Sheng Hu
    Haiming Cheng
    Journal of Radioanalytical and Nuclear Chemistry, 2016, 307 : 1471 - 1479
  • [25] Recovery of uranium(VI) from aqueous solution by amidoxime functionalized wool fibers
    Yin, Zhonglong
    Xiong, Jie
    Chen, Min
    Hu, Sheng
    Cheng, Haiming
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2016, 307 (02) : 1471 - 1479
  • [26] Removal of uranium(VI) from aqueous solution using graphene oxide and its amine-functionalized composite
    Shujuan Liu
    Song Li
    Hanxue Zhang
    Lipeng Wu
    Lei Sun
    Jianguo Ma
    Journal of Radioanalytical and Nuclear Chemistry, 2016, 309 : 607 - 614
  • [27] Removal of uranium(VI) from aqueous solution using graphene oxide and its amine-functionalized composite
    Liu, Shujuan
    Li, Song
    Zhang, Hanxue
    Wu, Lipeng
    Sun, Lei
    Ma, Jianguo
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2016, 309 (02) : 607 - 614
  • [28] A novel activated sludge-graphene oxide composites for the removal of uranium(VI) from aqueous solutions
    Zhao, Changsong
    Liu, Jun
    Yuan, Guoyuan
    Liu, Jian
    Zhang, Hailing
    Yang, Jijun
    Yang, Yuanyou
    Liu, Ning
    Sun, Qun
    Liao, Jiali
    JOURNAL OF MOLECULAR LIQUIDS, 2018, 271 : 786 - 794
  • [29] Removal of Pb(II) from aqueous solutions by graphene oxide aerogels
    Tabrizi, N. S.
    Zamani, S.
    WATER SCIENCE AND TECHNOLOGY, 2016, 74 (01) : 256 - 265
  • [30] Highly Efficient Removal of Uranium(VI) from Wastewater by Polyamidoxime/Polyethyleneimine Magnetic Graphene Oxide
    Dai, Zhongran
    Sun, Yusu
    Zhang, Hui
    Ding, Dexin
    Li, Le
    JOURNAL OF CHEMICAL AND ENGINEERING DATA, 2019, 64 (12): : 5797 - 5805