Theory of optical second-harmonic and sum-frequency scattering from arbitrarily shaped particles

被引：55

作者：

de Beer, Alex G. F. ^{[1
]}

Roke, Sylvie ^{[1
,2
]}

Dadap, Jerry I. ^{[3
]}

机构：

[1] Max Planck Inst Met Res, D-70569 Stuttgart, Germany

[2] Ecole Polytech Fed Lausanne, Sch Engn, Inst Bioengn, CH-1015 Lausanne, Switzerland

[3] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA

来源：

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS | 2011年 / 28卷 / 06期

基金：

欧洲研究理事会;

关键词：

CENTROSYMMETRIC MATERIAL; COLLOIDAL PARTICLES; SPHERICAL-PARTICLES; RAYLEIGH-SCATTERING; LIGHT-SCATTERING; GENERATION; SURFACE; SPECTROSCOPY; NANOPARTICLES; NANOCRYSTALS;

D O I：

10.1364/JOSAB.28.001374

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We present a theoretical framework for the generation and scattering of second-harmonic and sum-frequency light from the surface of particles of arbitrary shape in the limit of low index of refraction contrast. For homogeneous and isotropic surfaces, light scattering can be described by a finite set of scattering functions. Selection rules regarding these scattering functions are presented. We also find that the scattering functions associated with achiral and chiral surfaces are directly related to the bulk and surface linear optical form factors, respectively. Finally, we derive explicit expressions for particles of ellipsoidal shape, for which we calculate angular scattering patterns as a function of particle orientation and for ensembles of particles. (C) 2011 Optical Society of America

引用

页码：1374 / 1384

页数：11

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