Inward propagating chemical waves in a single-phase reaction-diffusion system

被引:29
|
作者
Shao, Xin [1 ]
Wu, Yabi [1 ]
Zhang, Jinzhong [1 ]
Wang, Hongli [1 ,2 ,3 ]
Ouyang, Qi [1 ,2 ,3 ]
机构
[1] Peking Univ, Dept Phys, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China
[2] Peking Univ, Beijing Hong Kong Singapore Joint Ctr Nonlinear &, Beijing 100871, Peoples R China
[3] Peking Univ, Ctr Theoret Biol, Beijing 100871, Peoples R China
关键词
D O I
10.1103/PhysRevLett.100.198304
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report our experimental and theoretical studies of inwardly propagating chemical waves (antiwaves) in a single-phase reaction-diffusion (RD) system. The experiment was conducted in an open spatial reactor using chlorite-iodide-malonic acid reaction. When the system was set to near Hopf bifurcation point, antiwaves appeared spontaneously, as predicted using both the reaction-diffusion (RD) equation and the complex Ginzburg-Landau equation (CGLE). Antiwaves change to ordinary waves when the system was moved away from the Hopf onset, which still agreed with RD simulations but could not be predicted by CGLE. We thus witnessed a new type of antiwave-wave exchange. Our analysis showed that this exchange occurred when the CGLE broke down as the system was far from the Hopf onset.
引用
收藏
页数:4
相关论文
共 50 条
  • [31] Reaction-diffusion waves in coupled isothermal autocatalytic chemical systems
    Metcalf, M.J.
    Merkin, J.H.
    Scott, S.K.
    1600, Publ by Oxford Univ Press, Oxford, United Kingdom (51):
  • [32] THE EXISTENCE OF SPIRAL WAVES IN AN OSCILLATORY REACTION-DIFFUSION SYSTEM
    PAULLET, J
    ERMENTROUT, B
    TROY, W
    SIAM JOURNAL ON APPLIED MATHEMATICS, 1994, 54 (05) : 1386 - 1401
  • [33] Modulated standing waves in a short reaction-diffusion system
    Dolnik, M
    Zhabotinsky, AM
    Epstein, IR
    JOURNAL OF PHYSICAL CHEMISTRY, 1996, 100 (16): : 6604 - 6607
  • [34] Chemical waves in reaction-diffusion networks of small organic molecules
    Paikar, Arpita
    Li, Xiuxiu
    Avram, Liat
    Smith, Barbara S.
    Suto, Istvan
    Horvath, Dezso
    Rennert, Elisabeth
    Qiu, Yuqing
    Toth, Agota
    Vaikuntanathan, Suriyanarayanan
    Semenov, Sergey N.
    CHEMICAL SCIENCE, 2025, 16 (02) : 659 - 669
  • [35] Reaction-diffusion waves in biology
    Volpert, V.
    Petrovskii, S.
    PHYSICS OF LIFE REVIEWS, 2009, 6 (04) : 267 - 310
  • [36] Flames and reaction-diffusion waves
    Clavin, P.
    Materials Science Forum, 1994, 155-5 : 445 - 446
  • [37] Resonant phase patterns in a reaction-diffusion system
    Lin, AL
    Bertram, M
    Martinez, K
    Swinney, HL
    Ardelea, A
    Carey, GF
    PHYSICAL REVIEW LETTERS, 2000, 84 (18) : 4240 - 4243
  • [39] Reaction-diffusion waves in mesospheric photochemical system with horizontal turbulent diffusion
    Kulikov, M.Yu.
    Feigin, A.M.
    Izvestiya Akademii Nauk. Ser. Fizicheskaya, 2004, 68 (12): : 1796 - 1803
  • [40] Field theory of propagating reaction-diffusion fronts
    Escudero, C
    PHYSICAL REVIEW E, 2004, 70 (04)