Uniform Distribution of Pd on GO-C Catalysts for Enhancing the Performance of Air Cathode Microbial Fuel Cell

被引:8
|
作者
Wang, Jingzhen [1 ,2 ]
Mu, Kaijie [2 ]
Zhao, Xuedong [2 ]
Luo, Dianliang [2 ]
Yu, Xiaodi [2 ]
Li, Wenpeng [3 ,4 ]
Chu, Jie [5 ]
Yang, Jing [6 ]
Yang, Qinzheng [1 ,2 ]
机构
[1] Qilu Univ Technol, Shandong Acad Sci, State Key Lab Biobased Mat & Green Papermaking, Jinan 250353, Peoples R China
[2] Qilu Univ Technol, Shandong Acad Sci, Dept Bioengn, Jinan 250353, Peoples R China
[3] Qilu Univ Technol, Shandong Acad Sci, Engn & Technol Ctr Electrochem, Sch Chem & Chem Engn, Jinan 250353, Peoples R China
[4] Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Shandong Key Lab Biochem Anal, Qingdao 266042, Peoples R China
[5] Qilu Univ Technol, Shandong Acad Sci, Biol Inst, Jinan 250103, Peoples R China
[6] Qilu Univ Technol, Shandong Acad Sci, Sch Elect & Informat Engn, Dept Phys, Jinan 250353, Peoples R China
基金
中国国家自然科学基金;
关键词
oxygen reduction reaction; microbial fuel cell; air cathode; OXYGEN REDUCTION REACTION; SUPPORTED PD; CARBON; ELECTROCATALYSTS; NANOPARTICLES; PALLADIUM; BLACK; ELECTRODE; FE;
D O I
10.3390/catal11080888
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Metal, as a high-performance electrode catalyst, is a research hotspot in the construction of a high-performance microbial fuel cell (MFC). However, metal catalyst nanoparticles and their dispersed carriers are prone to aggregation, producing catalytic electrodes with inferior qualities. In this study, Pd is uniformly dispersed on the graphene framework supported by carbon black to form nanocomposite catalysts (Pd/GO-C catalysts). The effect of the palladium loading amount in the catalyst on the catalytic performance of the air cathode was further studied. The optimized metal loading afforded a reduced resistance and improved accessibility of Pd particles for the ORR. The maximum current output of the 0.250 Pd (mg/cm(2)) MFC was 1645 mA/m(2), which is 4.2-fold higher than that of the carbon paper cathode. Overall, our findings provide a novel protocol for the preparation of high-efficient ORR catalyst for MFCs.
引用
收藏
页数:11
相关论文
共 50 条
  • [41] Performance and microbial ecology of air-cathode microbial fuel cells with layered electrode assemblies
    Butler, Caitlyn S.
    Nerenberg, Robert
    [J]. APPLIED MICROBIOLOGY AND BIOTECHNOLOGY, 2010, 86 (05) : 1399 - 1408
  • [42] Improved power and long term performance of microbial fuel cell with Fe-N-C catalyst in air-breathing cathode
    Gajda, Iwona
    Greenman, John
    Santoro, Carlo
    Serov, Alexey
    Melhuish, Chris
    Atanassov, Plamen
    Ieropoulos, Ioannis A.
    [J]. ENERGY, 2018, 144 : 1073 - 1079
  • [43] Performance and microbial ecology of air-cathode microbial fuel cells with layered electrode assemblies
    Caitlyn S. Butler
    Robert Nerenberg
    [J]. Applied Microbiology and Biotechnology, 2010, 86 : 1399 - 1408
  • [44] The performance of activated carbon treated with H3PO4 at 80 °C in the air-cathode microbial fuel cell
    Chen, Zhihao
    Li, Kexun
    Zhang, Peng
    Pu, Liangtao
    Zhang, Xi
    Fu, Zhou
    [J]. CHEMICAL ENGINEERING JOURNAL, 2015, 259 : 820 - 826
  • [45] Enhancing the performance of microbial fuel cell using a carbon-fiber-brush air cathode with low-cost mushroom Ganoderma laccase enzyme
    Lin, Chi-Wen
    Wu, Chih-Hung
    Lin, Yi-Ying
    Liu, Shu-Hui
    Chang, Shih-Hsien
    [J]. JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS, 2018, 85 : 115 - 120
  • [46] Application of Biogenic TiO2 Nanoparticles as ORR Catalysts on Cathode for Enhanced Performance of Microbial Fuel Cell
    Kumar, Ankit
    Siddiqui, Tabassum
    Pandit, Soumya
    Roy, Arpita
    Gacem, Amel
    Souwaileh, Abdullah Al
    Mathuriya, Abhilasha Singh
    Fatma, Tasneem
    Sharma, Promila
    Rustagi, Sarvesh
    Yadav, Krishna Kumar
    Jeon, Byong-Hun
    Park, Hyun-Kyung
    [J]. CATALYSTS, 2023, 13 (06)
  • [47] Bioelectrogeneic performance of air-cathode microbial fuel cells with diesel contaminants
    Zafar, Zargona
    Naz, Sarwat
    Malik, Noshaba Hassan
    Ahmed, Fayyaz
    Ali, Naeem
    [J]. FUEL, 2024, 355
  • [48] Effect of nitrate on the performance of single chamber air cathode microbial fuel cells
    Sukkasem, Chontisa
    Xu, Shoutao
    Park, Sunhwa
    Boonsawang, Piyarat
    Liu, Hong
    [J]. WATER RESEARCH, 2008, 42 (19) : 4743 - 4750
  • [49] Hybrid Biofuel Cell: Microbial Fuel Cell with an Enzymatic Air-Breathing Cathode
    Higgins, Scott R.
    Lau, Carolin
    Atanassov, Plamen
    Minteer, Shelley D.
    Cooney, Michael J.
    [J]. ACS CATALYSIS, 2011, 1 (09): : 994 - 997
  • [50] N-doped GO cathode catalyst boosting capacity of denitrification for air-cathode microbial fuel cell by shifting microbial community composition in treating marine wastewater
    Li, Xinyi
    Huang, Yangtian
    Lu, Yubiao
    Jia, Tianbo
    Wang, Jianxin
    Li, Peng
    [J]. JOURNAL OF WATER PROCESS ENGINEERING, 2023, 53