Flow reversal reactor for the catalytic combustion of lean methane mixtures

This paper describes an experimental investigation of a pilot scale reverse flow reactor for the catalytic destruction of lean mixtures of methane in air. It was found that using reverse flow it was possible maintain elevated reactor temperatures which were capable of achieving high methane conversion of methane in air streams at methane concentrations as low as 0.19% by volume. The space velocity, cycle time and feed concentration are all important parameters that govern the operation of the reactor. Control of these parameters is important to prevent the trapping of the thermal energy within the catalyst bed, which can limit the amount of energy that can be usefully extracted from the reactor. (C) 2003 Elsevier B.V. All rights reserved.