Synergetic effect of piezoelectricity and heterojunction on photocatalytic performance

被引:15
|
作者
Yin, Xin [1 ]
Wu, Wen [1 ]
Zhang, Fangshu [2 ]
Li, Ling [2 ]
Kou, Jiahui [1 ,2 ,3 ]
Lu, Chunhua [1 ,2 ,3 ]
机构
[1] Nanjing Tech Univ, Coll Mat Sci & Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 210009, Peoples R China
[2] Nanjing Tech Univ, Jiangsu Collaborat Innovat Ctr Adv Inorgan Funct, Nanjing 210009, Peoples R China
[3] Nanjing Tech Univ, Jiangsu Natl Synerget Innovat Ctr Adv Mat SICAM, Nanjing 210009, Peoples R China
基金
中国国家自然科学基金;
关键词
Piezoelectric; Photocatalysis; Heterojunction; g-C3N4; MoS2; VISIBLE-LIGHT; H-2; EVOLUTION; REDUCTION; COMPOSITE; CO2; NANOWIRES; EFFICIENT;
D O I
10.1016/j.jphotochem.2020.112661
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The less-than-ideal photogenerated electron-hole behaviors is one of the significant reasons for the low photocatalytic efficiency. In this work, organic piezoelectric material, PVDF, was used to restrain the recombination of photogenerated electron-hole of MoS2/g-C3N4 heterojunction photocatalyst, which aimed to enhance the photocatalytic performance. After being compounded with the PVDF, the photocatalytic activity of MoS2/g-C3N4 heterojunction can be increased by 66.8 %, which showed that the MoS2/g-C3N4 heterojunction had an excellent enhancement effect on the photocatalytic efficiency of the composite film. Compared with the pristine g-C3N4 photocatalyst piezoelectric film, the piezoelectric effect of heterojunction piezoelectric films varies with the different amounts of MoS2. Among these different piezoelectric films, the 10-M-CN-P film possess highest photocatalytic performance, possibly due to the best synergistical effect of piezoelectricity and heterojunction.
引用
收藏
页数:8
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