Universal Scaling of Intrinsic Resistivity in Two-Dimensional Metallic Borophene

被引：23

作者：

Zhang, Jin ^{[1
,2
,3
]}

Zhang, Jia ^{[1
,2
,3
]}

Zhou, Liujiang ^{[4
,5
]}

Cheng, Cai ^{[1
,2
,3
]}

Lian, Chao ^{[1
,2
,3
]}

Liu, Jian ^{[1
,2
,3
]}

Tretiak, Sergei ^{[4
,5
]}

Lischner, Johannes ^{[6
,7
,8
]}

Giustino, Feliciano ^{[9
]}

Meng, Sheng ^{[1
,2
,3
]}

机构：

[1] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China

[2] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China

[3] Univ Chinese Acad Sci, Sch Phys Sci, Beijing 100049, Peoples R China

[4] Los Alamos Natl Lab, Theoret Div, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA

[5] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA

[6] Imperial Coll London, Dept Mat, London SW7 2AZ, England

[7] Imperial Coll London, Dept Phys, London SW7 2AZ, England

[8] Imperial Coll London, Thomas Young Ctr Theory & Simulat Mat, London SW7 2AZ, England

[9] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2018年 / 57卷 / 17期

基金：

中国国家自然科学基金;

关键词：

Bloch-Gruneisen model; borophene; electron-phonon coupling; intrinsic electrical resistivity; BORON;

D O I：

10.1002/anie.201800087

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Two-dimensional boron sheets (borophenes) have been successfully synthesized in experiments and are expected to exhibit intriguing transport properties. A comprehensive first-principles study is reported of the intrinsic electrical resistivity of emerging borophene structures. The resistivity is highly dependent on different polymorphs and electron densities of borophene. Interestingly, a universal behavior of the intrinsic resistivity is well-described using the Bloch-Gruneisen model. In contrast to graphene and conventional metals, the intrinsic resistivity of borophenes can be easily tuned by adjusting carrier densities, while the Bloch-Gruneisen temperature is nearly fixed at 100K. This work suggests that monolayer boron can serve as intriguing platform for realizing tunable two-dimensional electronic devices.

引用

页码：4585 / 4589

页数：5

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