Temperature dependence of pressure-driven water permeation through membranes consisting of vertically-aligned double-walled carbon nanotube arrays

被引：7
|
作者：
Shirahama, Shiho [1 ]
Zhang, Shaoling [1 ]
Aiba, Motohiro [1 ,2 ]
Inoue, Hirotaka [3 ]
Hada, Masaki [3 ,4 ]
Hayashi, Yasuhiko [3 ,4 ]
Hata, Kenjiro [5 ]
Tsuruoka, Shuji [6 ]
Matsumoto, Hidetoshi [1 ]
机构：
[1] Tokyo Inst Technol, Dept Mat Sci & Engn, Meguro Ku, Mail Box S8-27,2-12-1 Ookayama, Tokyo 1528552, Japan
[2] Nagoya Municipal Ind Res Inst, Atsuta Ku, 3-4-41 Rokuban, Nagoya, Aichi 4560058, Japan
[3] Okayama Univ, Grad Sch Nat Sci & Technol, Okayama 7008530, Japan
[4] Tokyo Inst Technol, Inst Innovat Res, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528550, Japan
[5] YOUTEC Co Ltd, 5-7-3 Oze, Yashio, Saitama 3400822, Japan
[6] Shinshu Univ, Inst Carbon Sci & Technol, 4-17-1 Wakasato, Nagano 3808553, Japan
来源：
CARBON | 2019年 / 146卷
基金：
日本科学技术振兴机构;
关键词：
TRANSPORT; FABRICATION;
D O I：
10.1016/j.carbon.2019.02.031
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We explore the temperature dependence of pressure-driven water permeation through membranes consisting of a vertically aligned double-walled carbon nanotube (VA DWCNT) array. The prepared membrane with CNT inner diameter of 3.9 nm exhibits no water permeation below the critical temperature of 26 degrees C, after which water permeability is first observed and increases with temperatures > 26 degrees C. Further, the critical temperature decreases to 18 degrees C when the CNT inner diameter increases to 6.0 nm. The water permeation in the CNT-confined space exhibits activation energy transitions around room temperature, thereby suggesting that the confined water molecules in CNTs exhibit plural ordered structures. (C) 2019 Elsevier Ltd. All rights reserved.
引用
收藏
页码：785 / 788
页数：4
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