Enhanced water flux in vertically aligned carbon nanotube arrays and polyethersulfone composite membranes

被引:60
|
作者
Li, Shaoyun [1 ,3 ]
Liao, Gaomin [1 ,3 ]
Liu, Zhipeng [1 ,3 ]
Pan, Yuanyuan [1 ,3 ]
Wu, Qiang [1 ,2 ]
Weng, Yuyan [3 ]
Zhang, Xiaohua [3 ]
Yang, Zhaohui [3 ]
Tsui, Ophelia K. C. [4 ]
机构
[1] Soochow Univ, Dept Polymer Sci & Engn, Coll Chem Chem Engn & Mat Sci, Suzhou 215006, Peoples R China
[2] Soochow Univ, Dept Phys, Ctr Soft Condensed Matter Phys & Interdisciplinar, Suzhou 215006, Peoples R China
[3] Soochow Univ, Ctr Soft Condensed Matter Phys & Interdisciplinar, Suzhou 215006, Peoples R China
[4] Boston Univ, Dept Phys, Boston, MA 02134 USA
基金
美国国家科学基金会; 中国国家自然科学基金;
关键词
NANOCOMPOSITE MEMBRANES; MASS-TRANSPORT; FABRICATION; PURIFICATION; DESALINATION; TECHNOLOGY;
D O I
10.1039/c4ta02119c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We describe a novel preparation concept for a unique class of high-flux ultra-filtration membrane comprising a pre-aligned multi-walled carbon nanotube (MWCNT) array and polyethersulfone (PES). This membrane contains vertically aligned CNTs uniformly distributed inside a PES matrix. The vertically oriented water transportation pathway along the CNTs is verified to facilitate a dramatic enhancement in the water flux through the membrane. The water transportation speed increases about 3 times over the simply mixed CNT/PES membrane with random orientation and more than 10 times over the pure PES membrane under the same pressure load. Low working pressures as well as good retention properties enable this new composite membrane to be an ideal candidate for the future design of a highly efficient filtration membrane. This facile technique can potentially be applied to other filtration membrane systems to improve the separation efficiency.
引用
收藏
页码:12171 / 12176
页数:6
相关论文
共 50 条
  • [1] Effect of vertically aligned carbon nanotube density on the water flux and salt rejection in desalination membranes
    Trivedi, Samarth
    Alameh, Kamal
    SPRINGERPLUS, 2016, 5
  • [2] Vertically Aligned Carbon Nanotube Membranes: Water Purification and Beyond
    Lee, Jeong Hoon
    Kim, Han-Shin
    Yun, Eun-Tae
    Ham, So-Young
    Park, Jeong-Hoon
    Ahn, Chang Hoon
    Lee, Sang Hyup
    Park, Hee-Deung
    MEMBRANES, 2020, 10 (10) : 1 - 31
  • [3] Order in vertically aligned carbon nanotube arrays
    Wang, H
    Xu, Z
    Eres, G
    APPLIED PHYSICS LETTERS, 2006, 88 (21)
  • [4] Gas transport in vertically-aligned carbon nanotube/parylene composite membranes
    Zhang, Lei
    Zhao, Bin
    Wang, Xianying
    Liang, Youxuan
    Qiu, Hanxun
    Zheng, Guangping
    Yang, Junhe
    CARBON, 2014, 66 : 11 - 17
  • [5] Surface properties of vertically aligned carbon nanotube arrays
    Wirth, C. T.
    Hofmann, S.
    Robertson, J.
    DIAMOND AND RELATED MATERIALS, 2008, 17 (7-10) : 1518 - 1524
  • [6] Growth Mechanism of Vertically Aligned Carbon Nanotube Arrays
    Zhang, Ji-cheng
    Tang, Yong-jian
    Yi, Yong
    Zhou, Min-jie
    Ma, Kang-fu
    Wu, Wei-dong
    Wang, Chao-yang
    Zhao, Yon
    Luo, Bing-chi
    Wang, Zhuo
    CHINESE JOURNAL OF CHEMICAL PHYSICS, 2015, 28 (05) : 617 - 622
  • [7] Tribological properties of vertically aligned carbon nanotube arrays
    Schaber, Clemens F.
    Heinlein, Thorsten
    Keeley, Gareth
    Schneider, Joerg J.
    Gorb, Stanislav N.
    CARBON, 2015, 94 : 396 - 404
  • [8] Modelling clustering of vertically aligned carbon nanotube arrays
    Schaber, Clemens F.
    Filippov, Alexander E.
    Heinlein, Thorsten
    Schneider, Joerg J.
    Gorb, Stanislav N.
    INTERFACE FOCUS, 2015, 5 (04)
  • [9] Electrochemical modification of vertically aligned carbon nanotube arrays
    Ye, X. R.
    Chen, L. H.
    Wang, C.
    Aubuchon, J. F.
    Chen, I. C.
    Gapin, A. I.
    Talbot, J. B.
    Jin, S.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (26): : 12938 - 12942
  • [10] Tribological properties of vertically aligned carbon nanotube arrays and carbon nanotube sponge
    Chen, Jie
    Wang, Wen
    Zhang, Sheng
    AIP ADVANCES, 2020, 10 (12)