A 1D Co(II) coordination polymer based on semi-rigid bis(thiabendazole) and butane-1,2,3,4-tetracarboxylic acid linkers: synthesis, crystal structure, fluorescence sensing and photocatalytic properties

被引：13
|
作者：
Xiao, Qing-Qing [1 ]
Liu, Dong [1 ]
Li, Yue-Hua [1 ]
Cui, Guang-Hua [1 ]
机构：
[1] North China Univ Sci & Technol, Coll Chem Engn, Hebei Key Lab Environm Photocatalyt & Electrocata, 21 Bohai Rd, Tangshan 063210, Hebei, Peoples R China
来源：
POLYHEDRON | 2019年 / 166卷
基金：
中国国家自然科学基金;
关键词：
Co-based coordination polymer; Crystal structure; Fluorescence sensing; Fe3+; Photocatalytic property; METAL-ORGANIC FRAMEWORK; FLEXIBLE BIS(THIABENDAZOLE); SONOCHEMICAL SYNTHESIS; TOPOLOGICAL ANALYSIS; METHYLENE-BLUE; FE(III) IONS; TURN-ON; SENSOR; DEGRADATION; PHOTODEGRADATION;
D O I：
10.1016/j.poly.2019.03.027
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A Co(II)-based ternary coordination polymer with formula {[Co(BTC)(0.5)(L)(H2O)]center dot 3H2O}(n) (NCST-2, NCST = North China University of Science and Technology) was constructed from 1,2-bis(thiabendazol-1-ylmethyl)benzene (L) and butane-1,2,3,4-tetracarboxylic acid (H4BTC) under hydrothermal conditions. NCST-2 features a one-dimensional zigzag chain, which is further extended through O-H center dot center dot center dot O hydrogen bond and pi center dot center dot center dot pi stacking interactions into a three-dimensional supramolecular network. NCST-2 exhibits highly selective and recyclable performance for the fluorescence sensing of Fe3+ in aqueous solution with a linear detection range of 0-400 mu M and a detection limit of 0.12 mu M. NCST-2 displays high photocatalytic activities for degrading methylene blue (MB) under UV irradiation. The possible mechanism of the photodegradation towards MB was investigated in detail. (C) 2019 Elsevier Ltd. All rights reserved.
引用
收藏
页码：65 / 72
页数：8
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