Preparation of Tetraethylenepentamine Modified Magnetic Graphene Oxide for Adsorption of Dyes from Aqueous Solution

被引:8
|
作者
Tang, Xiaosheng [1 ,2 ,3 ]
Tang, Ping [4 ,5 ]
Liu, Liangliang [4 ]
机构
[1] Hubei Normal Univ, Hubei Key Lab Edible Wild Plants Conservat & Util, Huangshi 435002, Hubei, Peoples R China
[2] Hubei Normal Univ, Natl Demonstrat Ctr Expt Biol Educ, Huangshi 435002, Hubei, Peoples R China
[3] Hubei Normal Univ, Coll Life Sci, Hubei Key Lab Pollutant Anal & Reuse Technol, Huangshi 435002, Hubei, Peoples R China
[4] Chinese Acad Agr Sci, Inst Bast Fiber Crops, Changsha 410205, Hunan, Peoples R China
[5] Hubei Polytech Univ, Sch Environm Sci & Engn, Hubei Key Lab Mine Environm Pollut Control & Reme, Huangshi 435003, Hubei, Peoples R China
关键词
adsorption; dye; graphene oxide; magnetic nanoparticles; tetraethylenepentamine; ACID RED 18; EFFICIENT ADSORPTION; ANIONIC DYES; REMOVAL; NANOCOMPOSITE; COMPOSITE;
D O I
10.21577/0103-5053.20170145
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this study, tetraethylenepentamine modified magnetic graphene oxide nanomaterial (TMGO) was prepared and characterized by transmission electron microscopy (TEM), Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, thermogravimetric analysis (TGA), X-ray photoelectron spectroscopy (XPS) and vibration sample magnetometer (VSM). All the characterizations proved that the modification and preparation of TMGO were successful. The TMGO nanomaterial was used in the adsorption of Acid Red 18 (AR) in aqueous solution. The parameters like pH of solution, adsorption kinetics and isotherms were all investigated. The results indicated that the TMGO nanomaterial had satisfied adsorption ability and the maximum adsorption capacity was 524.2 mg g(-1) at 45 degrees C and pH 6. The adsorption capacity remained at 91.8% of the initial value after five cycles. The adsorption process with AR was found through fitting the pseudo-second-order kinetics equations and the Freundlich adsorption model. The experimental results demonstrated that the TMGO nanomaterial could be rapidly extracted from the medium and had a good adsorption ability to remove dyes in wastewater.
引用
收藏
页码:334 / 342
页数:9
相关论文
共 50 条
  • [41] Surface modified mesoporous silica polymer nanocomposites for adsorption of dyes from aqueous solution
    Sharma, Ankita
    Dubey, Amit
    JOURNAL OF POROUS MATERIALS, 2017, 24 (02) : 429 - 435
  • [42] Surface modified mesoporous silica polymer nanocomposites for adsorption of dyes from aqueous solution
    Ankita Sharma
    Amit Dubey
    Journal of Porous Materials, 2017, 24 : 429 - 435
  • [43] The adsorption of basic dyes from aqueous solution on modified peat-resin particle
    Sun, QY
    Yang, LZ
    WATER RESEARCH, 2003, 37 (07) : 1535 - 1544
  • [44] Preparation of ionic liquid modified graphene composites and their adsorption mechanism of arsenic (V) in aqueous solution
    Yingli Li
    Keyi Xiang
    Guangfei Qu
    Rui Li
    Environmental Science and Pollution Research, 2024, 31 : 16401 - 16412
  • [45] Adsorption of atrazine from aqueous solution using magnetic grapheme oxide
    Zhang, Xiaojun
    Ma, Xiaoguo
    Shu, Weiheng
    Peng, Junbiao
    PROCEEDINGS OF THE 2017 6TH INTERNATIONAL CONFERENCE ON MEASUREMENT, INSTRUMENTATION AND AUTOMATION (ICMIA 2017), 2017, 154 : 586 - 590
  • [46] Preparation of ionic liquid modified graphene composites and their adsorption mechanism of arsenic (V) in aqueous solution
    Li, Yingli
    Xiang, Keyi
    Qu, Guangfei
    Li, Rui
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2024, 31 (11) : 16401 - 16412
  • [47] Adsorption of atrazine from aqueous solution using magnetic grapheme oxide
    Zhang, Xiaojun
    Ma, Xiaoguo
    Shu, Weiheng
    Peng, Junbiao
    PROCEEDINGS OF THE 2017 6TH INTERNATIONAL CONFERENCE ON MEASUREMENT, INSTRUMENTATION AND AUTOMATION (ICMIA 2017), 2017, 154 : 511 - 515
  • [48] Preparation of magnetic graphene oxide/chitosan composite beads for effective removal of heavy metals and dyes from aqueous solutions
    Thi Thanh Nhi Le
    Van Thuan Le
    My Uyen Dao
    Quang Vinh Nguyen
    Thi Thu Vu
    Minh Hiep Nguyen
    Dai Lam Tran
    Hoang Sinh Le
    CHEMICAL ENGINEERING COMMUNICATIONS, 2019, 206 (10) : 1337 - 1352
  • [49] Simultaneous removal of Cd(II) and ionic dyes from aqueous solution using magnetic graphene oxide nanocomposite as an adsorbent
    Deng, Jiu-Hua
    Zhang, Xiu-Rong
    Zeng, Guang-Ming
    Gong, Ji-Lai
    Niu, Qiu-Ya
    Liang, Jie
    CHEMICAL ENGINEERING JOURNAL, 2013, 226 : 189 - 200
  • [50] Synthesis of polyethylenimine/graphene oxide for the adsorption of U(VI) from aqueous solution
    Liu, Hongjuan
    Zhou, Yuancheng
    Yang, Yibo
    Zou, Ke
    Wu, Renjie
    Xia, Ke
    Xie, Shuibo
    APPLIED SURFACE SCIENCE, 2019, 471 : 88 - 95