Spatial distribution of enhanced optical fields in one-dimensional linear arrays of gold nanoparticles studied by scanning near-field optical microscopy

被引:18
|
作者
Shimada, Toru [1 ]
Imura, Kohei [2 ,3 ]
Okamoto, Hiromi [4 ,5 ]
Kitajima, Masahiro [6 ]
机构
[1] Hirosaki Univ, Fac Educ, Dept Sci, Hirosaki, Aomori 0368560, Japan
[2] Waseda Univ, Sch Adv Sci & Engn, Dept Chem & Biochem, Shinjuku Ku, Okubo, Tokyo 1698555, Japan
[3] Japan Sci & Technol Agcy, PRESTO, Kawaguchi, Saitama 3320012, Japan
[4] Inst Mol Sci, Okazaki, Aichi 4448585, Japan
[5] Grad Univ Adv Studies, Okazaki, Aichi 4448585, Japan
[6] Natl Def Acad Japan, Sch Appl Sci, Dept Appl Phys, Yokosuka, Kanagawa 2398686, Japan
基金
日本学术振兴会;
关键词
RAMAN-ACTIVE SITES; VISUALIZATION; LOCALIZATION; SPECTRA; ENERGY; CHAINS; MODES;
D O I
10.1039/c2cp43128a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We visualized the enhanced optical field distributions in one-dimensional linear array structures of gold nanospheres by using scanning near-field optical microscopy. The characteristic field distribution depends on the chain length of the one-dimensional structures. The distribution of optical field is reproduced qualitatively by model calculations based upon finite-difference time-domain (FDTD) method. From the analysis, we have found that the characteristic distribution of the enhanced field arises from interparticle interactions, which cause propagation of the plasmon excitation in the inner part of the linear array, and trapping of it by a localized mode at the edges.
引用
收藏
页码:4265 / 4269
页数:5
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