Recent advances and future prospect in catalysts for oxidative coupling of methane to ethylene: A review

被引：106

作者：

Gambo, Y. ^{[1
]}

Jalil, A. A. ^{[1
,2
]}

Triwahyono, S. ^{[3
]}

Abdulrasheed, A. A. ^{[1
,4
]}

机构：

[1] Univ Teknol Malaysia, Fac Chem & Energy Engn, Dept Chem Engn, Utm Johor Bahru 81310, Johor, Malaysia

[2] Univ Teknol Malaysia, Inst Future Energy, Ctr Hydrogen Energy, Utm Johor Bahru 81310, Johor, Malaysia

[3] Univ Teknol Malaysia, Fac Sci, Dept Chem, Utm Johor Bahru 81310, Johor, Malaysia

[4] Abubakar Tafawa Balewa Univ, Dept Chem Engn, PMB 0248, Bauchi, Bauchi State, Nigeria

来源：

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY | 2018年 / 59卷

关键词：

Oxidative coupling of methane; Electrophilic lattice oxygen; Oxide reducibility; Oxygen vacancy; Active sites; FISCHER-TROPSCH SYNTHESIS; SILICA NANOPARTICLES MSN; OXIDE OXYGEN CARRIERS; HYDROGEN-PRODUCTION; MEMBRANE REACTOR; HETEROGENEOUS CATALYSIS; STATISTICAL-ANALYSIS; LA2O3; CATALYSTS; CARBON-DIOXIDE; KINETIC-MODEL;

D O I：

10.1016/j.jiec.2017.10.027

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Despite its inherent constraints which hindered significant improvement in the process catalytically, the oxidative coupling of methane (OCM) remains an indispensable prospective approach for converting methane directly into vital chemicals such as ethylene. Recently, there is an upsurge in research effort towards better understanding of the oxidative coupling of methane process in terms of its mechanism, catalyst design and synthesis. This review discusses recent advances in crucial aspects related to the catalyst such as active sites, oxygen vacancy, acid-base property, surface oxide reducibility, oxide support interaction, and prospects of nanowires with the aim to improve the performance of the OCM process. (C) 2017 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.

引用

页码：218 / 229

页数：12

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