Recent advances in the selective catalytic reduction of NOx with NH3 on Cu-Chabazite catalysts

被引:295
|
作者
Wang, Jihui [1 ]
Zhao, Huawang [1 ]
Haller, Gary [2 ]
Li, Yongdan [1 ,2 ]
机构
[1] Tianjin Univ, Sch Chem Engn, State Key Lab Chem Engn,Tianjin Key Lab Appl Cata, Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China
[2] Yale Univ, Dept Chem & Environm Engn, 9 Hillhouse Ave, New Haven, CT 06511 USA
关键词
Selective catalytic reduction of NOx with ammonia; Cu-Chabazite structured zeolite; Hydrothermal stability; Reaction mechanism; Preparation; STATE ION-EXCHANGE; CU-SAPO-34 MONOLITH CATALYST; CU/SSZ-13 NH3-SCR CATALYSTS; ONE-POT SYNTHESIS; CU/SAPO-34; CATALYSTS; LOW-TEMPERATURE; ACTIVE-SITES; HYDROTHERMAL STABILITY; CU-SSZ-13; CATALYST; MOLECULAR-SIEVES;
D O I
10.1016/j.apcatb.2016.09.024
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The development of Cu-chabazite (CHA) catalysts, i.e. Cu-SSZ-13 and Cu-SAPO-34, represents a significant technology breakthrough for the removal of NOx by selective catalytic reduction (SCR) with ammonia. Cu-CHA catalysts show an excellent hydrothermal stability towards high temperature aging and wide active temperature windows for the ammonia SCR reaction. This work summarizes the recent progress in the development of the Cu-CHA catalysts for the NH3-SCR reaction. The state of Cu in the reaction and the preparation methods on the catalytic performance are discussed. The advances in the understanding of the reaction mechanism are reviewed. The hydrothermal stability of the typical Cu-CHA catalysts are compared. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:346 / 354
页数:9
相关论文
共 50 条
  • [31] Preparation and performance of modified sintering dust catalysts for selective catalytic reduction of NOx with NH3
    Cheng, Qiao
    Fang, De
    Wu, Zhichao
    Zhang, Wan
    Wang, Qibo
    Xie, Junlin
    He, Feng
    [J]. MATERIALS RESEARCH EXPRESS, 2019, 6 (07):
  • [32] Vanadium-bearing steel slag catalysts for the selective catalytic reduction of NOx by NH3
    Xing, Yi
    Guo, Zefeng
    Su, Wei
    Zhang, Hui
    Chen, Jing
    Tian, Jinglei
    Yuan, Jichao
    Wu, Di
    [J]. NEW JOURNAL OF CHEMISTRY, 2022, 46 (31) : 14944 - 14957
  • [33] Enhanced activity of tungsten doped CeAlOX catalysts for the selective catalytic reduction of NOx with NH3
    Zhang, Peng
    Li, Kaihui
    Lei, Qingduo
    [J]. REACTION KINETICS MECHANISMS AND CATALYSIS, 2015, 116 (02) : 523 - 533
  • [34] Hydrothermal and sulfur aging of CeTi/CeWTi catalysts for selective catalytic reduction of NOx with NH3
    Lei Chen
    Ding Wang
    Jiadao Wang
    Duan Weng
    Li Cao
    [J]. Journal of Rare Earths, 2019, 37 (08) : 829 - 836
  • [35] Mechanistic Investigation into the Effect of Sulfuration on the FeW Catalysts for the Selective Catalytic Reduction of NOx with NH3
    Wang, Hui
    Qu, Zhenping
    Dong, Shicheng
    Tang, Chen
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (08) : 7017 - 7028
  • [36] Selective Catalytic Reduction (SCR) of NOx with NH3 on Sb-promoted VWTi Catalysts
    Kim, Su Bin
    Choi, Gyeong Ryun
    Shin, Jung Hun
    Hong, Sung Chang
    [J]. APPLIED CHEMISTRY FOR ENGINEERING, 2021, 32 (01): : 35 - 41
  • [37] The selective catalytic reduction of NOx with NH3 over titania supported rhenium oxide catalysts
    Wachs, IE
    Deo, G
    Andreini, A
    Vuurman, MA
    deBoer, M
    [J]. JOURNAL OF CATALYSIS, 1996, 160 (02) : 322 - 325
  • [38] Enhanced activity of tungsten doped CeAlOX catalysts for the selective catalytic reduction of NOx with NH3
    Peng Zhang
    Kaihui Li
    Qingduo Lei
    [J]. Reaction Kinetics, Mechanisms and Catalysis, 2015, 116 : 523 - 533
  • [39] Hydrothermal and sulfur aging of CeTi/CeWTi catalysts for selective catalytic reduction of NOx with NH3
    Chen, Lei
    Wang, Ding
    Wang, Jiadao
    Weng, Duan
    Cao, Li
    [J]. JOURNAL OF RARE EARTHS, 2019, 37 (08) : 829 - 836
  • [40] Sb-Containing Metal Oxide Catalysts for the Selective Catalytic Reduction of NOx with NH3
    Xu, Qian
    Liu, Dandan
    Wang, Chuchu
    Zhan, Wangcheng
    Guo, Yanglong
    Guo, Yun
    Wang, Li
    Ke, Qingping
    Ha, Minh Ngoc
    [J]. CATALYSTS, 2020, 10 (10) : 1 - 17