Coincidence imaging of polyatomic molecules via laser-induced Coulomb explosion

被引:34
|
作者
Gagnon, J. [1 ,2 ]
Lee, Kevin F. [2 ,3 ]
Rayner, D. M. [2 ]
Corkum, P. B. [1 ,2 ,3 ]
Bhardwaj, V. R. [1 ]
机构
[1] Univ Ottawa, Dept Phys, Ottawa, ON K1N 6N5, Canada
[2] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada
[3] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
关键词
D O I
10.1088/0953-4075/41/21/215104
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We extend laser-induced Coulomb explosion imaging to retrieve the structure of the five-atom dichloromethane (CH2Cl2) molecule by developing coincidence imaging and geometry optimization techniques. By detecting all five atoms in coincidence, we show that, from the measured velocity vectors, the geometry of the molecules can be reconstructed.
引用
收藏
页数:6
相关论文
共 50 条
  • [21] Observation of laser-induced electronic structure in oriented polyatomic molecules
    P. M. Kraus
    O. I. Tolstikhin
    D. Baykusheva
    A. Rupenyan
    J. Schneider
    C. Z. Bisgaard
    T. Morishita
    F. Jensen
    L. B. Madsen
    H. J. Wörner
    Nature Communications, 6
  • [22] Experimental evidence of excited multicharged atomic fragments coming from laser-induced Coulomb explosion of molecules
    Quaglia, L
    Cornaggia, C
    PHYSICAL REVIEW LETTERS, 2000, 84 (20) : 4565 - 4568
  • [23] Laser-induced suppression of the Coulomb explosions of diatomic molecules
    Smirnova, O
    Ivanov, MY
    LASER PHYSICS, 2003, 13 (07) : 975 - 984
  • [24] COULOMB EXPLOSION IMAGING OF SMALL MOLECULES
    VAGER, Z
    NAAMAN, R
    KANTER, EP
    SCIENCE, 1989, 244 (4903) : 426 - 431
  • [25] Ultrafast Coulomb explosion imaging of molecules
    Cornaggia, C.
    LASER PHYSICS, 2009, 19 (08) : 1660 - 1670
  • [26] LASER-INDUCED DESORPTION OF POLYATOMIC-MOLECULES WITH A CO2-LASER
    SEEBAUER, EG
    KONG, ACF
    SCHMIDT, LD
    APPLIED SURFACE SCIENCE, 1987, 29 (03) : 380 - 390
  • [27] ULTRAFAST LASER-INDUCED COULOMB EXPLOSION OF CLUSTERS WITH HIGH CHARGE STATES
    PURNELL, J
    SNYDER, EM
    WEI, S
    CASTLEMAN, AW
    CHEMICAL PHYSICS LETTERS, 1994, 229 (4-5) : 333 - 339
  • [28] Laser-induced Coulomb explosion, geometry modification and reorientation of carbon dioxide
    Bryant, WA
    Sanderson, JH
    El-Zein, A
    Newell, WR
    Taday, PF
    Langley, AJ
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2000, 33 (04) : 745 - 766
  • [29] Breast cancer therapy by laser-induced Coulomb explosion of gold nanoparticles
    Muhammad Gul Bahar Ashiq
    Mohammad Alam Saeed
    Bashir Ahmad Tahir
    Noorddin Ibrahim
    Muhammad Nadeem
    Chinese Journal of Cancer Research, 2013, 25 (06) : 756 - 761
  • [30] Breast cancer therapy by laser-induced Coulomb explosion of gold nanoparticles
    Ashiq, Muhammad Gul Bahar
    Saeed, Mohammad Alain
    Tahir, Bashir Ahmad
    Ibrahim, Noorddin
    Nadeem, Muhammad
    CHINESE JOURNAL OF CANCER RESEARCH, 2013, 25 (06) : 756 - 761