Nonlinear Fano profiles in the optical second-harmonic generation from silver nanoparticles

被引:11
|
作者
Butet, J. [1 ]
Bachelier, G. [1 ]
Russier-Antoine, I. [1 ]
Bertorelle, F. [1 ]
Mosset, A. [1 ]
Lascoux, N. [1 ]
Jonin, C. [1 ]
Benichou, E. [1 ]
Brevet, P. -F. [1 ]
机构
[1] Univ Lyon 1, Lab Spectrometrie Ion & Mol, CNRS, UMR 5579, F-69622 Villeurbanne, France
关键词
RAYLEIGH-SCATTERING;
D O I
10.1103/PhysRevB.86.075430
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The resonance effects on the optical second-harmonic generation from 140-nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences between the broad dipolar and narrow octupolar surface plasmon resonances leads to nonlinear Fano profiles that can be externally controlled by the incident polarization angle. These profiles are responsible for the plasmon-induced suppression of the second harmonic generation.
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页数:5
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