Tungstate doped TiO2-SiO2 aerogels for preferential photocatalytic degradation of methamphetamine in seizure samples containing caffeine under simulated sunlight

被引:13
|
作者
Li, Yizhou [1 ]
Yang, Yepeng [1 ]
Yang, Peisong [1 ]
Jiang, Liang [1 ]
Wang, Wei [1 ]
He, Jiao [1 ]
Chen, Yongjuan [1 ]
Wang, Jiaqiang [1 ]
机构
[1] Yunnan Univ, Natl Ctr Int Res Photoelect & Energy Mat, Yunnan Prov Engn Res Ctr Photocatalyt Treatment I, Sch Chem Sci & Technol,Sch Mat & Energy, Kunming 650091, Yunnan, Peoples R China
基金
中国国家自然科学基金;
关键词
Methamphetamine; Preferentially photocatalytic degradation; Tungstate; Aerogels; TiO2; ILLICIT DRUGS; OXIDATION; TITANIA; REMOVAL; PHARMACEUTICALS; ENHANCEMENT; COMPLEXES; PRODUCTS;
D O I
10.1016/j.catcom.2020.106121
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Tungstate doped TiO2-SiO2 aerogels (W/TiO2-SiO2) was synthesized and photocatalytic degraded methamphetamine (MAT) preferentially in seizure samples which containing caffeine. As a control, TiO2 (P25) photocatalytic degraded both MAT and caffeine simultaneously. The degradation rate of MAT under simulated sunlight for TiO2 (P25), TiO2-SiO2 aerogels, W/TiO2 and W/TiO2-SiO2 are 28.1%, 64.2%, 74.1% and 98.8% within 60 min. The photocatalytic efficiency of W/TiO2-SiO2 for degradation of MAT is 7.0, 4.4 and 1.9 times higher than TiO2 (P25), TiO2-SiO2 aerogels and W/TiO2. The enhanced photocatalytic performance of W/TiO2-SiO2 could be attributed to increase the adsorption of MAT induced by tungstate-doping.
引用
收藏
页数:5
相关论文
共 50 条
  • [31] Simulated Sunlight Irradiation Based Photocatalytic Degradation of Acrylonitrile by Sn-F Co-doped TiO2/SiO2Nano Powder Catalyst
    Hanliang Li
    Shiyu Miao
    Lu Qiu
    Bandna Bharti
    Feng Ouyang
    Journal of Harbin Institute of Technology(New Series), 2021, 28 (01) : 12 - 19
  • [32] High Efficiency Degradation of Tetracycline Antibiotic with TiO2-SiO2 Photocatalyst under Low Power of Simulated Solar Light Irradiation
    Thi-Ngoc-Bich Duong
    Minh-Vien Le
    11TH REGIONAL CONFERENCE ON CHEMICAL ENGINEERING (RCCHE 2018), 2019, 2085
  • [33] THE PHOTOCATALYTIC ACTIVITY OF N-DOPED TiO2 UNDER SUNLIGHT
    Liu, Liquing
    Peng, Bing
    Chai, Liyuan
    Li, Guoliang
    Liu, Yunchao
    TMS 2009 138TH ANNUAL MEETING & EXHIBITION - SUPPLEMENTAL PROCEEDINGS, VOL 1: MATERIALS PROCESSING AND PROPERTIES, 2009, : 7 - 11
  • [34] Sol-gel synthesis of sodium silicate and titanium oxychloride based TiO2-SiO2 aerogels and their photocatalytic property under UV irradiation
    Kim, You Na
    Shao, Godlisten N.
    Jeon, Sung Jeong
    Imran, S. M.
    Sarawade, Pradip B.
    Kim, Hee Taik
    CHEMICAL ENGINEERING JOURNAL, 2013, 231 : 502 - 511
  • [35] Enhancing efficiency and photocatalytic activity of TiO2-SiO2 by combination of glycerol for MO degradation in continuous reactor under solar irradiation
    Hoang, Nhung Thi-Tuyet
    Tran, Anh Thi-Kim
    Le, Thanh-An
    Nguyen, D. Duc
    JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2021, 9 (05):
  • [36] Photocatalytic degradation of phenol in water under simulated sunlight by an ultrathin MgO coated Ag/TiO2 nanocomposite
    Scott, Tyler
    Zhao, Huilei
    Deng, Wei
    Feng, Xuhui
    Li, Ying
    CHEMOSPHERE, 2019, 216 : 1 - 8
  • [37] Adsorption and photocatalytic degradation of gas-phase UDMH under simulated sunlight by AgBr/TiO2/rGA
    Hou Ruomeng
    Jia Ying
    Lv Xiaomeng
    Huang Yuanzheng
    Shen Keke
    RSC ADVANCES, 2021, 11 (21) : 12583 - 12594
  • [38] Photocatalytic activity of AgBr/TiO2 in water under simulated sunlight irradiation
    Zang, Yujing
    Farnood, Ramin
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2008, 79 (04) : 334 - 340
  • [39] Enhanced photocatalytic degradation of the herbicide 2,4-dichlorophenoxyacetic acid by Pt/TiO2-SiO2 nanocomposites
    Gonzalez, Alberto Estrella
    Asomoza, Maximiliano
    Solis, Silvia
    Sanchez, Miguel A. Garcia
    Cipagauta-Diaz, Sandra
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2020, 131 (01) : 489 - 503
  • [40] Study on the photocatalytic activity of rare earth Gd-doped TiO2 nanocrystallites under simulated sunlight
    Cai, He-Shan
    Liu, Guo-Guang
    Li, Xiao-Xia
    Yingxiang Kexue yu Guanghuaxue/Imaging Science and Photochemistry, 2008, 26 (03): : 238 - 243