Tungstate doped TiO2-SiO2 aerogels for preferential photocatalytic degradation of methamphetamine in seizure samples containing caffeine under simulated sunlight

被引:13
|
作者
Li, Yizhou [1 ]
Yang, Yepeng [1 ]
Yang, Peisong [1 ]
Jiang, Liang [1 ]
Wang, Wei [1 ]
He, Jiao [1 ]
Chen, Yongjuan [1 ]
Wang, Jiaqiang [1 ]
机构
[1] Yunnan Univ, Natl Ctr Int Res Photoelect & Energy Mat, Yunnan Prov Engn Res Ctr Photocatalyt Treatment I, Sch Chem Sci & Technol,Sch Mat & Energy, Kunming 650091, Yunnan, Peoples R China
基金
中国国家自然科学基金;
关键词
Methamphetamine; Preferentially photocatalytic degradation; Tungstate; Aerogels; TiO2; ILLICIT DRUGS; OXIDATION; TITANIA; REMOVAL; PHARMACEUTICALS; ENHANCEMENT; COMPLEXES; PRODUCTS;
D O I
10.1016/j.catcom.2020.106121
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Tungstate doped TiO2-SiO2 aerogels (W/TiO2-SiO2) was synthesized and photocatalytic degraded methamphetamine (MAT) preferentially in seizure samples which containing caffeine. As a control, TiO2 (P25) photocatalytic degraded both MAT and caffeine simultaneously. The degradation rate of MAT under simulated sunlight for TiO2 (P25), TiO2-SiO2 aerogels, W/TiO2 and W/TiO2-SiO2 are 28.1%, 64.2%, 74.1% and 98.8% within 60 min. The photocatalytic efficiency of W/TiO2-SiO2 for degradation of MAT is 7.0, 4.4 and 1.9 times higher than TiO2 (P25), TiO2-SiO2 aerogels and W/TiO2. The enhanced photocatalytic performance of W/TiO2-SiO2 could be attributed to increase the adsorption of MAT induced by tungstate-doping.
引用
收藏
页数:5
相关论文
共 50 条
  • [1] Preparation and photocatalytic activity of TiO2-SiO2 binary aerogels
    Deng, ZS
    Wang, J
    Zhang, YL
    Weng, ZN
    Zhang, Z
    Zhou, B
    Shen, J
    Cheng, LY
    NANOSTRUCTURED MATERIALS, 1999, 11 (08): : 1313 - 1318
  • [2] Photocatalytic degradation of flumequine by N-doped TiO2 catalysts under simulated sunlight
    Zeng, Xiaolan
    Sun, Xiaozi
    Wang, Yan
    ENVIRONMENTAL ENGINEERING RESEARCH, 2021, 26 (06)
  • [3] Efficient degradation of doxycycline and ofloxacin in an aqueous environment using Fe and Cu doped TiO2-SiO2 photocatalyst under sunlight
    Rani, Sonam
    Garg, Alok
    Singh, Neetu
    ENVIRONMENTAL ENGINEERING RESEARCH, 2022, 27 (04)
  • [4] Photocatalytic degradation and kinetics of Methyl orange with Bi-doped TiO2 under simulated sunlight
    Rong, Chuan
    Dong, Xiaoli
    Ma, Chun
    Zhang, Xinxin
    Shi, Fei
    BIOTECHNOLOGY, CHEMICAL AND MATERIALS ENGINEERING II, PTS 1 AND 2, 2013, 641-642 : 229 - 232
  • [5] Hollow TiO2-SiO2 Nanospheres for Photocatalytic Degradation of Organic Dyes
    Xu, Dongming
    Yu, Haomiao
    Qin, Yang
    Di, Yang
    Jia, Hongbing
    Li, Fengsheng
    Liu, Jie
    ACS APPLIED NANO MATERIALS, 2024, 7 (03) : 2630 - 2638
  • [6] Preparation of mesoporous TiO2-SiO2 and photocatalytic degradation of black liquor
    Lin Huiliang
    Zhou Guowei
    Liu Ying
    Meng Qinghai
    Xu Huiying
    New Technologies in Non-Wood Fiber Pulping and Papermaking, 2006, : 358 - 362
  • [7] Photocatalytic degradation of phenol by hydrothermally synthesized TiO2-SiO2 mixed oxides
    Kibombo, Harrison
    Zhao, Dan
    Budhi, Sridhar
    Gonshorowski, Andra
    Koodali, Ranjit T.
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2010, 239
  • [8] PHOTOCATALYTIC DEGRADATION OF PYRENE IN POROUS Pt/TiO2-SiO2 PHOTOCATALYST SUSPENSION UNDER UV IRRADIATION
    Luo, Zhaohui
    Katayama-Hirayama, Keiko
    Hirayama, Kimiaki
    Akitsu, Tetsuya
    Kaneko, Hidehiro
    NANO, 2008, 3 (05) : 317 - 322
  • [9] Cu2+ doped TiO2-SiO2 with photonic crystal structure for synergistic enhancement of photocatalytic degradation under visible light irradiation
    Wu, Yuanting
    Liu, Tiantian
    Hei, Xiping
    Liu, Qiujun
    Wang, Xiufeng
    NANOTECHNOLOGY, 2021, 32 (43)
  • [10] Design of Ag/ and Pt/TiO2-SiO2 nanomaterials for the photocatalytic degradation of phenol under solar irradiation
    Juan Matos
    Biviana Llano
    Ricmary Montaña
    Po S. Poon
    Maria C. Hidalgo
    Environmental Science and Pollution Research, 2018, 25 : 18894 - 18913