Catalytic Oxidation of NO on N-doped Carbon Materials at Low Temperature

被引:12
|
作者
Zou, Xiuyong [1 ]
Lou, Shifeng [1 ]
Yang, Chao [1 ]
Liu, Naiwang [1 ]
Wang, Xin [1 ]
Shi, Li [1 ]
Meng, Xuan [1 ]
机构
[1] East China Univ Sci & Technol, Int Joint Res Ctr Green Energy Chem Engn, Shanghai 200237, Peoples R China
基金
美国国家科学基金会;
关键词
Removal of NO; Activated carbon; Nitrogen doping; Catalytic oxidation; NITRIC-OXIDE NO; ACTIVATED CARBON; SURFACE-CHEMISTRY; NITROGEN FUNCTIONALITIES; REDUCTION; PERFORMANCE; GRAPHENE; TRANSFORMATION; COMPOSITES; ADSORPTION;
D O I
10.1007/s10562-020-03297-7
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
By hetero atom doping, a nitrogen-doped porous carbon was synthesized and applied to catalytic oxidation removal of NO. The synthesis conditions and NO removal process conditions of the modified carbon material were investigated, including calcination temperatures, impregnation amount, NO inlet concentration (100-500 ppm) and catalytic reaction temperature. The results showed that the dicyandiamide impregnation solution concentration of 0.5 M, and the calcination temperature of 600 degrees C performed the best in the preparation of structurally stable nitrogen-modified carbon. Due to the formation of a large number active centers of pyridine nitrogen (N-6) groups and graphitic nitrogen (N-Q) groups, the optimal conversion rate of NO could reach 67.2%. Graphic
引用
收藏
页码:487 / 496
页数:10
相关论文
共 50 条
  • [41] Thermal removal of partial nitrogen atoms in N-doped graphene for enhanced catalytic oxidation
    Zhao, Yang
    Wu, Di
    Chen, Ying
    Li, Yang
    Fan, Xiaobin
    Zhang, Fengbao
    Zhang, Guoliang
    Peng, Wenchao
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2021, 585 : 640 - 648
  • [42] N-Doped Porous Carbon Supported Au Nanoparticles for Benzyl Alcohol Oxidation
    Mao, Donglei
    Jia, Mingmin
    Qiu, Jianhao
    Zhang, Xiong-Fei
    Yao, Jianfeng
    CATALYSIS LETTERS, 2020, 150 (01) : 74 - 81
  • [43] Oxidation Evolution and Activity Origin of N-Doped Carbon in the Oxygen Reduction Reaction
    Wu, Jiaqi
    Cheng, Chuanqi
    Lu, Shanshan
    Zhang, Bin
    Shi, Yanmei
    TRANSACTIONS OF TIANJIN UNIVERSITY, 2024, 30 (04) : 369 - 379
  • [44] N-Doped Amorphous Carbon Supported Pd Catalysts for Methanol Electrocatalytic Oxidation
    Zhao Yan-Chun
    Zhan Lu
    Tian Jian-Niao
    Nie Su-Lian
    Ning Zhen
    ACTA PHYSICO-CHIMICA SINICA, 2011, 27 (01) : 91 - 96
  • [45] Ni/NiO heterojunction anchored on N-doped carbon for the enhanced methanol oxidation
    Guo, Ruihong
    Zhang, Yujuan
    Zhang, Xiutang
    Hu, Tuoping
    JOURNAL OF ALLOYS AND COMPOUNDS, 2023, 960
  • [46] Printing specific active sites for ORR and hydrazine oxidation on N-doped carbon
    Pereira, Guilherme M.
    Cellet, Thelma S. P.
    Winkler, Manuel E. G.
    Rubira, Adley F.
    Silva, Rafael
    MATERIALS CHEMISTRY AND PHYSICS, 2023, 307
  • [47] N-Doped Porous Carbon Supported Au Nanoparticles for Benzyl Alcohol Oxidation
    Donglei Mao
    Mingmin Jia
    Jianhao Qiu
    Xiong-Fei Zhang
    Jianfeng Yao
    Catalysis Letters, 2020, 150 : 74 - 81
  • [48] Oxidation Evolution and Activity Origin of N-Doped Carbon in the Oxygen Reduction Reaction
    Jiaqi Wu
    Chuanqi Cheng
    Shanshan Lu
    Bin Zhang
    Yanmei Shi
    Transactions of Tianjin University, 2024, 30 (04) : 369 - 379
  • [49] The Influence of Carbonization Temperature and KOH Activation Ratio on the Microporosity of N-doped Activated Carbon Materials and Their Supercapacitive Behaviors
    Son, Yeong-Rae
    Heo, Young-Jung
    Cho, Eun-A
    Park, Soo-Jin
    COMPOSITES RESEARCH, 2018, 31 (05): : 267 - 275
  • [50] N-doped carbon nanotubes for electrocatalysis
    Stevenson, Keith J.
    Wiggins-Camacho, Jaclyn
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2010, 239