Femtosecond nuclear motion of HCl probed by resonant x-ray Raman scattering in the Cl 1s region

被引：63

作者：

Simon, M

Journel, L

Guillemin, R

Stolte, WC

Minkov, I

Gel'mukhanov, F

Salek, P

Ågren, H

Carniato, S

Taïeb, R

Hudson, AC

Lindle, DW

机构：

[1] Lab Chim Phys Mat & Rayonnement, UMR 7614, F-75231 Paris 05, France

[2] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA

[3] Royal Inst Technol, S-10691 Stockholm, Sweden

来源：

PHYSICAL REVIEW A | 2006年 / 73卷 / 02期

关键词：

D O I：

10.1103/PhysRevA.73.020706

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Femtosecond dynamics are observed by resonant x-ray Raman scattering (RXS) after excitation along the dissociative Cl 1s -> 6 sigma(*) resonance of gas-phase HCl. The short core-hole lifetime results in a complete breakdown of the common nondispersive behavior of soft-x-ray transitions between parallel potentials. We evidence a general phenomenon of RXS in the hard-x-ray region: a complete quenching of vibrational broadening. This opens up a unique opportunity for superhigh resolution x-ray spectroscopy beyond vibrational and lifetime limitations.

引用

页数：4

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