MoS2 Quantum Dots-Modified Covalent Triazine-Based Frameworks for Enhanced Photocatalytic Hydrogen Evolution

被引：86
|
作者：
Jiang, Qianqian [1 ]
Sun, Long [1 ]
Bi, Jinhong [1 ,2 ]
Liang, Shijing [1 ,2 ]
Li, Liuyi [3 ]
Yu, Yan [3 ]
Wu, Ling [2 ]
机构：
[1] Fuzhou Univ, Dept Environm Sci & Engn, Minhou 350108, Fujian, Peoples R China
[2] Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Minhou 350108, Fujian, Peoples R China
[3] Fuzhou Univ, Key Lab Ecomat Adv Technol, Minhou 350108, Fujian, Peoples R China
来源：
CHEMSUSCHEM | 2018年 / 11卷 / 06期
基金：
中国国家自然科学基金;
关键词：
covalent organic frameworks; electron transfer; hydrogen evolution; quantum dots; photocatalysis; VISIBLE-LIGHT; EFFICIENT PHOTOCATALYST; CONJUGATED POLYMERS; FACILE SYNTHESIS; ONE-POT; WATER; COCATALYSTS; NANOSHEETS; PERFORMANCE; COMPOSITES;
D O I：
10.1002/cssc.201702220
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
MoS2 quantum dots (QDs)-modified covalent triazine-based framework (MoS2/CTF) composites are synthesized through an in situ photodeposition method. MoS2 QDs are well distributed and stabilized on the layers of CTFs by coordination of the frameworks to MoS2. The QDs-sheet interactions between MoS2 and CTFs facilitate interfacial charge transfer and separation. As a consequence, the composites exhibit outstanding photocatalytic activity and stability for hydrogen evolution under visible light irradiation (lambda >= 420 nm), that exceed those over pristine CTFs and MoS2-modified g-C3N4 (MoS2/g-C3N4) composite, making them promising materials for solar energy conversion.
引用
收藏
页码：1108 / 1113
页数：6
相关论文
共 50 条
  • [21] Hydrogen and CO2 storage in high surface area covalent triazine-based frameworks
    Deng, Q. -W.
    Ren, G. -Q.
    Li, Y. -J.
    Yang, L.
    Zhai, S. -L.
    Yu, T.
    Sun, L.
    Deng, W. -Q.
    Li, A.
    Zhou, Y. -H.
    [J]. MATERIALS TODAY ENERGY, 2020, 18
  • [22] Modulating electronic structure of triazine-based covalent organic frameworks for photocatalytic organic transformations
    Gu, Zhangjie
    Wang, Jinjian
    Shan, Zhen
    Wu, Miaomiao
    Liu, Tongtong
    Song, Liang
    Wang, Guixiang
    Ju, Xuehai
    Su, Jian
    Zhang, Gen
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2022, 10 (34) : 17624 - 17632
  • [23] Monolayer MoS2 quantum dots as catalysts for efficient hydrogen evolution
    Qiao, Wen
    Yan, Shiming
    Song, Xueyin
    Zhang, Xing
    Sun, Yuan
    Chen, Xing
    Zhong, Wei
    Du, Youwei
    [J]. RSC ADVANCES, 2015, 5 (118): : 97696 - 97701
  • [24] The O/S heteroatom effects of covalent triazine frameworks for photocatalytic hydrogen evolution
    Liu, Manying
    Yang, Kangni
    Li, Zhenyang
    Fan, Erchuang
    Fu, Huafeng
    Zhang, Like
    Zhang, Yange
    Zheng, Zhi
    [J]. CHEMICAL COMMUNICATIONS, 2021, 58 (01) : 92 - 95
  • [25] Size-controlled synthesis of CdS nanoparticles confined on covalent triazine-based frameworks for durable photocatalytic hydrogen evolution under visible light
    Wang, Dengke
    Li, Xiang
    Zheng, Ling-Ling
    Qin, Lu-Mei
    Li, Shuang
    Ye, Peng
    Li, Yan
    Zou, Jian-Ping
    [J]. NANOSCALE, 2018, 10 (41) : 19509 - 19516
  • [26] Tuning size of MoS2 in MoS2/graphene oxide heterostructures for enhanced photocatalytic hydrogen evolution
    Min Wang
    Xiuxun Han
    Yun Zhao
    Jiajia Li
    Peng Ju
    Zhaomin Hao
    [J]. Journal of Materials Science, 2018, 53 : 3603 - 3612
  • [27] Tuning size of MoS2 in MoS2/graphene oxide heterostructures for enhanced photocatalytic hydrogen evolution
    Wang, Min
    Han, Xiuxun
    Zhao, Yun
    Li, Jiajia
    Ju, Peng
    Hao, Zhaomin
    [J]. JOURNAL OF MATERIALS SCIENCE, 2018, 53 (05) : 3603 - 3612
  • [28] MoS2 quantum dots-modified porous β-Bi2O3 microspheres with enhanced visible-light-induced photocatalytic activity for Bisphenol A degradation and NO removal
    Mirabbos Hojamberdiev
    Gangqiang Zhu
    Huan Lu
    Mahesh Kumar
    Miaomiao Wang
    Jianzhi Gao
    [J]. Journal of Materials Science: Materials in Electronics, 2019, 30 : 2610 - 2621
  • [29] MoS2 quantum dots-modified porous -Bi2O3 microspheres with enhanced visible-light-induced photocatalytic activity for Bisphenol A degradation and NO removal
    Hojamberdiev, Mirabbos
    Zhu, Gangqiang
    Lu, Huan
    Kumar, Mahesh
    Wang, Miaomiao
    Gao, Jianzhi
    [J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2019, 30 (03) : 2610 - 2621
  • [30] Engineering single-atom catalysts on triazine-based covalent organic frameworks for enhanced photocatalytic performance in N2 reduction
    Chen, Meiyan
    Li, Qingyu
    Xu, Xinyue
    Liu, Diwen
    Ma, Zuju
    Li, Yanxia
    Zhang, Yanjie
    Li, Dejing
    Chen, Qiang
    Sa, Rongjian
    [J]. CHEMICAL ENGINEERING JOURNAL, 2024, 494
12345