Performance enhancement of methane dry reforming reaction for syngas production over Ir/Ce0.9La0.1O2-nanorods catalysts

被引：50
|
作者：
Wang, Fagen [1 ]
Wang, Yan [1 ]
Zhang, Linjia [1 ]
Zhu, Jiayin [1 ]
Han, Bolin [1 ]
Fan, Weiqiang [1 ]
Xu, Leilei [2 ]
Yu, Hao [3 ]
Cai, Weijie [4 ]
Li, Zhongcheng [5 ]
Deng, Zhiyong [6 ]
Shi, Weidong [1 ]
机构：
[1] Jiangsu Univ, Sch Chem & Chem Engn, 301 Xuefu Rd, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Nanjing 210044, Peoples R China
[3] Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Qingdao 266590, Peoples R China
[4] Dalian Polytech Univ, Fac Light Ind & Chem Engn, Dalian 116023, Peoples R China
[5] Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266042, Peoples R China
[6] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China
来源：
CATALYSIS TODAY | 2020年 / 355卷
基金：
中国博士后科学基金; 中国国家自然科学基金;
关键词：
Ce0.9La0.1O2; Nanorods; Methane dry reforming; Metal-support interaction; HYDROGEN-PRODUCTION; SHELL NANOCATALYSTS; DOPED CERIA; EFFICIENT; OXIDATION; ETHANOL; RH; NANOPARTICLES; MORPHOLOGY; STABILITY;
D O I：
10.1016/j.cattod.2019.06.067
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
Ir catalysts supported on Ce0.9La0.1O2 nanorods and nanoparticles were comparatively investigated for syngas production from methane dry reforming reaction. The exposure of active {110} and {100} crystal planes in the Ir/Ceo Ce0.9La0.1O2- nanorods catalysts contributed to the stronger redox property and more oxygen vacancy than those in the Ir/Ce0.9La0.1O2-nanoparticles catalysts. These advantages facilitated activation and transformation of methane and carbon dioxide, giving an enhanced performance of methane dry reforming reaction over the Ir/Ce0.9La0.1O2-nanorods catalysts. The work demonstrated significant influences of support morphologies in obtaining stable catalysts for methane dry reforming reaction.
引用
收藏
页码：502 / 511
页数：10
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