Dipyrrolo[2,3-b:2′,3′-e]pyrazine-2,6(1H,5H)-dione based conjugated polymers for ambipolar organic thin-film transistors

被引:47
|
作者
Hong, Wei [1 ,2 ]
Sun, Bin [1 ,2 ]
Yuen, Jonathan [1 ,2 ]
Li, Yuning [1 ,2 ]
Lu, Shaofeng [3 ]
Huang, Chun [3 ]
Facchetti, Antonio [3 ]
机构
[1] Univ Waterloo, Dept Chem Engn, Waterloo, ON N2L 3G1, Canada
[2] Univ Waterloo, Waterloo Inst Nanotechnol WIN, Waterloo, ON N2L 3G1, Canada
[3] Polyera Corp, Skokie, IL 60077 USA
关键词
FIELD-EFFECT TRANSISTORS; HIGH-MOBILITY; COPOLYMER; PERFORMANCE; TRANSPORT; HOLE;
D O I
10.1039/c2cc37266e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report two new low band-gap conjugated polymers containing dipyrrolo[2,3-b:2',3'-e]pyrazine-2,6(1H,5H)-dione (PzDP), PPzDPDP-BT and PPzDPDP-TT, both showing ambipolar transport in organic thin film transistors (OTFTs), with hole mobility up to 0.066 cm(2) V-1 s(-1), electron mobility up to 0.021 cm(2) V-1 s(-1), and high current on-to-off ratios of 10(5)-10(6).
引用
收藏
页码:484 / 486
页数:3
相关论文
共 50 条
  • [21] Synthesis of 6-amino-5-R2-7-(6-R1-4-oxo-3,4-dihydro-2-quinazolyl)- 5H-pyrrolo[2,3-b]-pyrazine-2,3-dicarbonitriles
    Volovenko Yu.M.
    Dubinina G.G.
    Chemistry of Heterocyclic Compounds, 2002, 38 (02) : 219 - 225
  • [22] 6-amino-2-phenylimidazo[4,5-e][1,3]diazepine-4,8(1H, 5H)-dione
    Chen, HM
    Hosmane, RS
    MOLECULES, 2000, 5 (07) : M164 - M164
  • [23] CRYSTAL-STRUCTURE OF 1,6-DIAMINOTETRAHYDROPYRROLO-[2,3-B]PYRROLE-2,5(1H,3H)-DIONE, C6H10N4O2
    ALVAREZLARENA, A
    PINIELLA, JF
    VICTORY, P
    BORRELL, JI
    BETI, C
    COMELLAS, L
    ZEITSCHRIFT FUR KRISTALLOGRAPHIE, 1993, 203 : 110 - 112
  • [24] Bis(2-oxoindolin-3-ylidene)-benzodifuran-dione and bithiophene-based conjugated polymers for high performance ambipolar organic thin-film transistors: the impact of substitution positions on bithiophene units
    Wang, Xiaohong
    Choi, Hyun Ho
    Zhang, Guobing
    Ding, Yunsheng
    Lu, Hongbo
    Cho, Kilwon
    Qiu, Longzhen
    JOURNAL OF MATERIALS CHEMISTRY C, 2016, 4 (26) : 6391 - 6400
  • [25] 1,1′,3,3′,5,5′-Hexamethylspiro[furo[2,3-d]pyrimidine-6(5H),5′-pyrimidine]-2,2′,4,4′,6′(1H,3H,1′H,3′H,5′H)-pentaone
    Pesyan, Nader Noroozi
    Rastgar, Saeed
    Hosseini, Yaser
    ACTA CRYSTALLOGRAPHICA SECTION E-STRUCTURE REPORTS ONLINE, 2009, 65 : O1444 - U3327
  • [26] PYROLYSIS AND PROPERTIES OF TRIS(2,3-EPOXYPROPYL)-1,3,5-TRIAZINE-2,4,6(1H,3H,5H)-TRIONE AND TRIS(2,3-EPOXY-3-METHYLPROPYL)-1,3,5-TRIAZINE-2,4,6(1H,3H,5H)-TRIONE
    SHIMASAKI, C
    TAKEUCHI, M
    TSUTUGUCHI, J
    SHIMIZU, K
    YAMAKAWA, H
    BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1985, 58 (08) : 2197 - 2202
  • [27] One-pot [1+1+1] synthesis of dithieno[2,3-b:3′,2′-d]thiophene (DTT) and their functionalized derivatives for organic thin-film transistors
    Chen, Ming-Chou
    Chiang, Yen-Ju
    Kim, Choongik
    Guo, Yue-Jhih
    Chen, Sheng-Yu
    Liang, You-Jhih
    Huang, Yu-Wen
    Hu, Tarng-Shiang
    Lee, Gene-Hsiang
    Facchetti, Antonio
    Marks, Tobin J.
    CHEMICAL COMMUNICATIONS, 2009, (14) : 1846 - 1848
  • [28] Diphenyl Derivatives of Dinaphtho[2,3-b:2′,3′-f]thieno[3,2-b]thiophene: Organic Semiconductors for Thermally Stable Thin-Film Transistors
    Kang, Myeong Jin
    Miyazaki, Eigo
    Osaka, Itaru
    Takimiya, Kazuo
    Nakao, Akiko
    ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (07) : 2331 - 2336
  • [29] (3E,8E)-3,8-Bis(2-oxoindolin-3-ylidene)naphtho-[1,2-b:5,6-b′]difuran-2,7(3H,8H)-dione (INDF) based polymers for organic thin-film transistors with highly balanced ambipolar charge transport characteristics
    Deng, Yunfeng
    Sun, Bin
    He, Yinghui
    Quinn, Jesse
    Guo, Chang
    Li, Yuning
    CHEMICAL COMMUNICATIONS, 2015, 51 (70) : 13515 - 13518
  • [30] DIHYDROINDOL-7(6H)-ONES AND 6,7-DIHYDROPYRROLO[2,3-C]AZEPINE-4,8(1H,5H)-DIONE
    KASUM, B
    PRAGER, RH
    TSOPELAS, C
    AUSTRALIAN JOURNAL OF CHEMISTRY, 1990, 43 (02) : 355 - 365