In situ synthesis of a series of lanthanide coordination polymers based on N-heterocyclic carboxylate ligands: Crystal structure and luminescence

被引：11

作者：

Wang, Qi ^{[1
]}

Fan, Yong ^{[1
]}

Song, Tianyou ^{[1
]}

Xu, Jianing ^{[1
]}

Wang, Jia ^{[1
]}

Chai, Juan ^{[1
]}

Liu, Yunling ^{[2
]}

Wang, Li ^{[1
]}

Zhang, Lirong ^{[1
]}

机构：

[1] Jilin Univ, Coll Chem, Changchun 130012, Jilin, Peoples R China

[2] Jilin Univ, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Jilin, Peoples R China

来源：

INORGANICA CHIMICA ACTA | 2015年 / 438卷

基金：

中国国家自然科学基金;

关键词：

Coordination polymer; In situ synthesis; Luminescence; Lanthanide; N-heterocyclic carboxylate ligands; METAL-ORGANIC FRAMEWORKS; AG(I) COMPLEXES; ACID; ARCHITECTURES; NETWORKS; CLUSTER; WATER; NETS;

D O I：

10.1016/j.ica.2015.08.033

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

A series of novel lanthanide coordination polymers (Ln-CPs) have been constructed by 2-(pyridin-2-yl-N-oxide)-1H-imidazole-4,5-dicarboxylate (H3POIDC) ligand, which derived from the partial oxidation of 2-(pyridin-2-yl)-1H-imidazole-4,5-dicarboxylate (H3PIDC) in situ reaction. Compounds 1-3 with the infinite left-and right-hand helices show 3D supramolecular structure constructing from 1D chains connecting each other through strong hydrogen-bond interactions. Compounds 4-7 show 2D layered structure with sql topology which are built from 4-connected nodes. Moreover, compounds 1-6 show strong luminescence emission in solid state, especially compound 1 exhibits obvious luminescence quenching for Hg2+ ion. (C) 2015 Elsevier B.V. All rights reserved.

引用

页码：128 / 134

页数：7

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