In situ synthesis of a series of lanthanide coordination polymers based on N-heterocyclic carboxylate ligands: Crystal structure and luminescence

被引：11
|
作者：
Wang, Qi [1 ]
Fan, Yong [1 ]
Song, Tianyou [1 ]
Xu, Jianing [1 ]
Wang, Jia [1 ]
Chai, Juan [1 ]
Liu, Yunling [2 ]
Wang, Li [1 ]
Zhang, Lirong [1 ]
机构：
[1] Jilin Univ, Coll Chem, Changchun 130012, Jilin, Peoples R China
[2] Jilin Univ, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Jilin, Peoples R China
来源：
INORGANICA CHIMICA ACTA | 2015年 / 438卷
基金：
中国国家自然科学基金;
关键词：
Coordination polymer; In situ synthesis; Luminescence; Lanthanide; N-heterocyclic carboxylate ligands; METAL-ORGANIC FRAMEWORKS; AG(I) COMPLEXES; ACID; ARCHITECTURES; NETWORKS; CLUSTER; WATER; NETS;
D O I：
10.1016/j.ica.2015.08.033
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A series of novel lanthanide coordination polymers (Ln-CPs) have been constructed by 2-(pyridin-2-yl-N-oxide)-1H-imidazole-4,5-dicarboxylate (H3POIDC) ligand, which derived from the partial oxidation of 2-(pyridin-2-yl)-1H-imidazole-4,5-dicarboxylate (H3PIDC) in situ reaction. Compounds 1-3 with the infinite left-and right-hand helices show 3D supramolecular structure constructing from 1D chains connecting each other through strong hydrogen-bond interactions. Compounds 4-7 show 2D layered structure with sql topology which are built from 4-connected nodes. Moreover, compounds 1-6 show strong luminescence emission in solid state, especially compound 1 exhibits obvious luminescence quenching for Hg2+ ion. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码：128 / 134
页数：7
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