Optimized Synthesis of Fe/N/C Cathode Catalysts for PEM Fuel Cells: A Matter of Iron-Ligand Coordination Strength

被引：179

作者：

Tian, Juan ^{[1
]}

Morozan, Adina ^{[2
]}

Sougrati, Moulay Tahar ^{[2
]}

Lefevre, Michel ^{[1
]}

Chenitz, Regis ^{[1
]}

Dodelet, Jean-Pol ^{[1
]}

Jones, Deborah ^{[2
]}

Jaouen, Frederic ^{[2
]}

机构：

[1] Inst Natl Rech Sci Energie Mat & Telecommun, Varennes, PQ J3X 1S2, Canada

[2] Univ Montpellier 2, Inst Charles Gerhardt Montpellier, F-34095 Montpellier, France

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 27期

基金：

加拿大自然科学与工程研究理事会;

关键词：

chelates; fuel cells; iron; UV; Vis spectroscopy; zeolites; OXYGEN REDUCTION REACTION; METAL-ORGANIC FRAMEWORKS; ELECTROCATALYSTS; COMPLEXES; STABILITY; IMIDAZOLE; ION;

D O I：

10.1002/anie.201303025

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

It's all in the detail: Highly active Fe/N/C catalysts for the oxygen-reduction reaction in polymer-electrolyte-membrane (PEM) fuel cells can be obtained from a precursor constructed from the zeolitic imidazolate framework ZIF-8 and an iron-ligand complex if, and only if, the displacement of Zn II ions from ZIF-8 by FeII ions is restricted (see picture; TPTZ=2,4,6-tris(2-pyridyl)-s-triazine). Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：6867 / 6870

页数：4

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