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Efficient Photoelectrochemical Water Splitting by g-C3N4/TiO2 Nanotube Array Heterostructures
被引:137
|作者:
Liu, Changhai
[1
]
Wang, Fang
[1
]
Zhang, Jin
[1
]
Wang, Ke
[1
]
Qiu, Yangyang
[1
]
Liang, Qian
[2
]
Chen, Zhidong
[2
]
机构:
[1] Changzhou Univ, Sch Mat Sci & Engn, Jiangsu Collaborat Innovat Ctr Photovolta Sci & E, Changzhou 213164, Jiangsu, Peoples R China
[2] Changzhou Univ, Sch Petrochem Engn, Changzhou 213164, Jiangsu, Peoples R China
基金:
中国国家自然科学基金;
关键词:
TiO2 nanotube arrays;
Graphitic carbon nitride (g-C3N4);
Heterojunction;
Photoelectrochemical;
Water splitting;
TIO2 NANOWIRE ARRAYS;
PHOTOCATALYTIC PERFORMANCE;
HETEROJUNCTIONS;
ANATASE;
GROWTH;
DEGRADATION;
FABRICATION;
COMPOSITES;
CONVERSION;
NANOSHEETS;
D O I:
10.1007/s40820-018-0192-6
中图分类号:
TB3 [工程材料学];
学科分类号:
0805 ;
080502 ;
摘要:
Well-ordered TiO2 nanotube arrays (TNTAs) decorated with graphitic carbon nitride (g-C3N4) were fabricated by anodic oxidization and calcination process. First, TNTAs were prepared via the anodic oxidation of Ti foil in glycerol solution containing fluorinion and 20% deionized water. Subsequently, g-C3N4 film was hydrothermally grown on TNTAs via the hydrogen-bonded cyanuric acid melamine supramolecular complex. The results showed that g-C3N4 was successfully decorated on the TNTAs and the g-C3N4/TNTAs served as an efficient and stable photoanode for photoelectrochemical water splitting. The facile deposition method enables the fabrication of efficient and low-cost photoanodes for renewable energy applications. [GRAPHICS]
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页码:1 / 13
页数:13
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