Study on the coloring mechanism of the Ru celadon glaze in the Northern Song Dynasty

被引：19

作者：

Shi, Pei ^{[1
]}

Wang, Fen ^{[1
]}

Zhang, Biao ^{[1
]}

Luo, Hongjie ^{[2
]}

Zhu, Jianfeng ^{[1
]}

Fei, Guiqiang ^{[3
]}

机构：

[1] Shaanxi Univ Sci & Technol, Shaanxi Key Lab Green Preparat & Functionalizat I, Sch Mat Sci & Engn, Xian 710021, Peoples R China

[2] Shanghai Univ, Res Inst Cultural Rel, Shanghai 200444, Peoples R China

[3] Shaanxi Univ Sci & Technol, Coll Chem & Chem Engn, Xian 710021, Peoples R China

来源：

CERAMICS INTERNATIONAL | 2020年 / 46卷 / 15期

基金：

中国国家自然科学基金;

关键词：

Ru Guan kiln; Qingliangsi; Celadon glaze; Northern Song Dynasty; Coloring mechanism; DIFFERENTIATION; CERAMICS; SPECTRA; WARE;

D O I：

10.1016/j.ceramint.2020.06.139

中图分类号：

TQ174 [陶瓷工业]; TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

The Ru kiln is one of the five most famous kilns in the Chinese Song Dynasty. To clarify the coloring mechanism of the Ru celadon glaze, the celadon samples from the Ru Guan kiln site of Qingliangsi were analyzed by spectrophotometer, X-ray fluorescence spectrum, Raman spectroscopy, scanning electron microscopy and X-ray photoelectron spectrum. The results indicated that the molar ratios of SiO2/Al2O3 and CaO/(CaO + Al2O3) affected the formation of micro-bubbles, anorthite crystals and phase separated structures. A large number of bubbles and anorthite crystals formed special glossiness and opacifying effect in the Ru celadon glaze. And then, dense phase separation droplets in the amorphous region were in short-range order, but their diameters (31-46 nm) were too small to form visible structural colors on glaze surfaces. Only "opal effect" was formed by the light scattering, which added the aesthetic feeling for the Ru celadon. Besides, the phase separation droplets intensified the segregation of iron, and thus deepened the chemical color and made the Ru celadon glaze appear green-blue. Due to the neutral to alkaline soil at the Ru Guan kiln site, the water in the soil and its corrosion on the Ru celadon glaze resulted in the formation of Si-OH bond.

引用

页码：23662 / 23668

页数：7

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