Isolating quantum coherence using coherent multi-dimensional spectroscopy with spectrally shaped pulses

被引：30
|
作者：
Tollerud, Jonathan O.
Hall, Christopher R.
Davis, Jeffrey A. [1 ]
机构：
[1] Swinburne Univ Technol, Ctr Quantum & Opt Sci, Hawthorn, Vic 3122, Australia
来源：
OPTICS EXPRESS | 2014年 / 22卷 / 06期
基金：
澳大利亚研究理事会;
关键词：
FOURIER-TRANSFORM SPECTROSCOPY; PHOTOSYNTHETIC MARINE-ALGAE; ENERGY-TRANSFER; PROTEIN; WELLS; TEMPERATURE; SYSTEMS; BEATS;
D O I：
10.1364/OE.22.006719
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
sWe demonstrate how spectral shaping in coherent multidimensional spectroscopy can isolate specific signal pathways and directly access quantitative details. By selectively exciting pathways involving a coherent superposition of exciton states we are able to identify, isolate and analyse weak coherent coupling between spatially separated excitons in an asymmetric double quantum well. Analysis of the isolated signal elucidates details of the coherent interactions between the spatially separated excitons. With a dynamic range exceeding 104 in electric field amplitude, this approach facilitates quantitative comparisons of different signal pathways and a comprehensive description of the electronic states and their interactions. (C) 2014 Optical Society of America
引用
收藏
页码：6719 / 6733
页数：15
相关论文
共 50 条
  • [21] Fast multi-dimensional Hadamard spectroscopy
    Kupce, E
    Freeman, R
    JOURNAL OF MAGNETIC RESONANCE, 2003, 163 (01) : 56 - 63
  • [22] MISC, an instrument for multi-dimensional spectroscopy
    Stolpe, F
    Kneer, F
    ASTRONOMY & ASTROPHYSICS SUPPLEMENT SERIES, 1998, 131 (01): : 181 - 185
  • [23] Quantum dynamics in condensed phases probed by multi-dimensional vibrational and NMR spectroscopy
    Tanimura, Yoshitaka
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2006, 231
  • [24] Power and spectrally efficient multi-dimensional WCDMA modem employing CPM
    Basilio, D. J.
    Linde, L. P.
    Maharaj, B. T.
    2007 AFRICON, VOLS 1-3, 2007, : 868 - 873
  • [25] Multi-dimensional coherent optical spectroscopy of semiconductor nanostructures: Collinear and non-collinear approaches
    Nardin, Gael
    Autry, Travis M.
    Moody, Galan
    Singh, Rohan
    Li, Hebin
    Cundiff, Steven T.
    JOURNAL OF APPLIED PHYSICS, 2015, 117 (11)
  • [26] Quantum control with multi-dimensional Gaussian quantum invariant
    Simsek, Selwyn
    Mintert, Florian
    QUANTUM, 2021, 5
  • [27] Quantum vision representations and multi-dimensional quantum transforms
    Li, Hai-Sheng
    Song, Shuxiang
    Fan, Ping
    Peng, Huiling
    Xia, Hai-ying
    Liang, Yan
    INFORMATION SCIENCES, 2019, 502 : 42 - 58
  • [28] Coherent quantum control of multiphoton transitions by shaped ultrashort optical pulses
    Meshulach, D
    Silberberg, Y
    PHYSICAL REVIEW A, 1999, 60 (02): : 1287 - 1292
  • [29] Femtosecond coherence spectroscopy using spectrally selective differential photodetection
    Rosca, F
    Ionascu, D
    Kumar, ATN
    Demidov, AA
    Champion, PM
    CHEMICAL PHYSICS LETTERS, 2001, 337 (1-3) : 107 - 116
  • [30] Multi-dimensional Hermite polynomials in quantum optics
    Kok, P
    Braunstein, SL
    JOURNAL OF PHYSICS A-MATHEMATICAL AND GENERAL, 2001, 34 (31): : 6185 - 6195
12345