Isolating quantum coherence using coherent multi-dimensional spectroscopy with spectrally shaped pulses

被引：30
|
作者：
Tollerud, Jonathan O.
Hall, Christopher R.
Davis, Jeffrey A. [1 ]
机构：
[1] Swinburne Univ Technol, Ctr Quantum & Opt Sci, Hawthorn, Vic 3122, Australia
来源：
OPTICS EXPRESS | 2014年 / 22卷 / 06期
基金：
澳大利亚研究理事会;
关键词：
FOURIER-TRANSFORM SPECTROSCOPY; PHOTOSYNTHETIC MARINE-ALGAE; ENERGY-TRANSFER; PROTEIN; WELLS; TEMPERATURE; SYSTEMS; BEATS;
D O I：
10.1364/OE.22.006719
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
sWe demonstrate how spectral shaping in coherent multidimensional spectroscopy can isolate specific signal pathways and directly access quantitative details. By selectively exciting pathways involving a coherent superposition of exciton states we are able to identify, isolate and analyse weak coherent coupling between spatially separated excitons in an asymmetric double quantum well. Analysis of the isolated signal elucidates details of the coherent interactions between the spatially separated excitons. With a dynamic range exceeding 104 in electric field amplitude, this approach facilitates quantitative comparisons of different signal pathways and a comprehensive description of the electronic states and their interactions. (C) 2014 Optical Society of America
引用
收藏
页码：6719 / 6733
页数：15
相关论文
共 50 条
  • [1] Isolating Quantum Coherence Using Coherent Multi-dimensional Spectroscopy with Spectrally Shaped Pulses
    Tollerud, Jonathan O.
    Hall, Christopher R.
    Davis, Jeffrey A.
    ULTRAFAST PHENOMENA XIX, 2015, 162 : 793 - 796
  • [2] Multi-dimensional coherent spectroscopy of CdSe colloidal quantum dots at cryogenic temperatures
    Liu, Albert
    Almeida, Diogo B.
    Ki, Wan
    Padilha, Lazaro A.
    Cundiff, Steven T.
    XXI INTERNATIONAL CONFERENCE ON ULTRAFAST PHENOMENA 2018 (UP 2018), 2019, 205
  • [3] Perspective: multi-dimensional coherent spectroscopy of perovskite nanocrystals
    Liu, Albert
    Almeida, Diogo B.
    Padilha, Lazaro A.
    Cundiff, Steven T.
    JOURNAL OF PHYSICS-MATERIALS, 2022, 5 (02):
  • [4] Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures
    Moody, Galan
    Cundiff, Steven T.
    ADVANCES IN PHYSICS-X, 2017, 2 (03): : 641 - 674
  • [5] Visualization and quantum control of light-accelerated condensates by terahertz multi-dimensional coherent spectroscopy
    Mootz, Martin
    Luo, Liang
    Wang, Jigang
    Perakis, Ilias E.
    COMMUNICATIONS PHYSICS, 2022, 5 (01)
  • [6] Visualization and quantum control of light-accelerated condensates by terahertz multi-dimensional coherent spectroscopy
    Martin Mootz
    Liang Luo
    Jigang Wang
    llias E. Perakis
    Communications Physics, 5
  • [7] Variational Quantum Demodulation for Coherent Optical Multi-Dimensional QAM
    Koike-Akino, Toshiaki
    Matsumine, Toshiki
    Wang, Ye
    Millar, David S.
    Kojima, Keisuke
    Parsons, Kieran
    2020 OPTICAL FIBER COMMUNICATIONS CONFERENCE AND EXPOSITION (OFC), 2020,
  • [8] Demonstration of a stable and flexible coherent multi-dimensional spectroscopy apparatus to study coherent coupling in asymmetric double quantum wells
    Tollerud, J. O.
    Richards, G.
    Tan, H. H.
    Jagadish, C.
    Davis, J. A.
    2012 CONFERENCE ON OPTOELECTRONIC AND MICROELECTRONIC MATERIALS AND DEVICES (COMMAD 2012), 2012, : 151 - +
  • [9] Multi-dimensional imaging by coherence measurement
    Yoshimori, Kyu
    INTERNATIONAL CONFERENCE ON PHOTONICS SOLUTIONS 2015, 2015, 9659
  • [10] ISOLATING OPENINGS FOR NEW PRODUCTS IN A MULTI-DIMENSIONAL SPACE
    MORGAN, N
    PURNELL, J
    JOURNAL OF THE MARKET RESEARCH SOCIETY, 1969, 11 (03): : 245 - 266
12345