Nonexponential Decay in the Quantum Dynamics of Nanosystems

被引:8
|
作者
Benderskii, V. A. [1 ]
Kats, E. I. [2 ,3 ]
机构
[1] Russian Acad Sci, Inst Problems Chem Phys, Chernogolovka 142432, Moscow Region, Russia
[2] Russian Acad Sci, LD Landau Theoret Phys Inst, Chernogolovka 142432, Moscow Region, Russia
[3] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
关键词
03.65.-w; 82.20.-w;
D O I
10.1134/S0021364008170116
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The quantum dynamical problem is solved fora system coupled to an equidistant-spectrum bath with the energy difference Omega between the neighboring levels n and n + 1 and the coupling matrix elements C-n(2) = C-2(1 + Delta(-2)n(2))(-1) constraining the energy interval comprising the bath states interacting with the system. The evolution in the strong-coupling limit is determined by two parameters, Gamma = pi C-2/Omega >> 1 and alpha = Gamma/Delta. If alpha not equal 0, then the decrease in the population in the initial cycle with a period of 2 pi/Omega is not exponential and the effective rate constant increases with time. The results qualitatively explain the appearance of nonexponential relaxation regimes for a dense-spectrum nanosystem and predict the possibility of the multiple recovery of the initial-state population.
引用
收藏
页码:338 / 341
页数:4
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