Rare metal-ion metathesis of a tetrahedral Zn(ii) core of a noncentrosymmetric (3,4)-connected 3D MOF

被引：7

作者：

Lee, Li-Wei ^{[1
,2
]}

Kao, Ya-Chuan ^{[1
]}

Chung, Mei-Ying ^{[1
]}

Chang, Bor-Chen ^{[3
]}

Lee, Gene-Hsiang ^{[4
]}

Peng, Shie-Ming ^{[4
]}

Wang, Chih-Min ^{[5
]}

Liu, Yen-Hsiang ^{[6
]}

Lee, Sheng-Long ^{[2
]}

Lu, Kuang-Lieh ^{[1
,2
]}

机构：

[1] Acad Sinica, Inst Chem, Taipei 115, Taiwan

[2] Natl Cent Univ, Inst Mat Sci & Engn, Taoyuan 320, Taiwan

[3] Natl Cent Univ, Dept Chem, Taoyuan 320, Taiwan

[4] Natl Taiwan Univ, Dept Chem, Taipei 107, Taiwan

[5] Natl Taiwan Ocean Univ, Dept Biosci & Biotechnol, Keelung 202, Taiwan

[6] Fu Jen Catholic Univ, Dept Chem, Taipei 242, Taiwan

来源：

DALTON TRANSACTIONS | 2019年 / 48卷 / 06期

关键词：

SINGLE-CRYSTAL TRANSFORMATION; ORGANIC FRAMEWORKS; POSTSYNTHETIC LIGAND; STEPWISE SYNTHESIS; CATION-EXCHANGE; ZINC PHOSPHITE; GAS UPTAKE; ADSORPTION; PHOTOLUMINESCENCE; CONSTRUCTION;

D O I：

10.1039/c8dt04472d

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

An SHG-active noncentrosymmetric (3,4)-connected Zn(II)-organic framework, {[Zn-2(4-abpt)(3,4-pydc)(2)]center dot 2DMAc center dot 3MeOH center dot H2O}(n) (1-Zn), was synthesized using a mixed-ligand system. The 1-Zn framework undergoes metal metathesis, with the complete exchange of the tetrahedrally coordinated Zn-II ions with Cu-II ions while retaining the integrity of the network.

引用

页码：1950 / 1954

页数：5

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