Concentration, sources and wet deposition of dissolved nitrogen and organic carbon in the Northern Indo-Gangetic Plain during monsoon

被引:14
|
作者
Bhattarai, Hemraj [1 ,2 ,6 ,8 ]
Tripathee, Lekhendra [3 ,6 ]
Kang, Shichang [3 ,4 ,5 ]
Sharma, Chhatra Mani [6 ]
Chen, Pengfei [3 ]
Guo, Junming [3 ]
Ghimire, Prakriti Sharma [3 ,7 ]
机构
[1] Chinese Univ Hong Kong, Earth Syst Sci Programme, Hong Kong, Peoples R China
[2] Chinese Univ Hong Kong, Grad Div Earth & Atmospher Sci, Hong Kong, Peoples R China
[3] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China
[4] Chinese Acad Sci, Key Lab Tibetan Environm Changes & Land Surface P, Inst Tibetan Plateau Res, Beijing 100101, Peoples R China
[5] Chinese Acad Sci, Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100085, Peoples R China
[6] Himalayan Environm Res Inst HERI, Kathmandu, Nepal
[7] Tribhuvan Univ, Cent Dept Environm Sci, Kathmandu, Nepal
[8] Kathmandu Ctr Res & Educ KCRE, Kathmandu, Nepal
来源
基金
中国国家自然科学基金;
关键词
Precipitation chemistry; Dissolved organic carbon; Total dissolved nitrogen; Major ions; Indo-Gangetic Plain; CHEMICAL-COMPOSITION; CENTRAL HIMALAYAS; IONIC COMPOSITION; URBAN SITE; PRECIPITATION CHEMISTRY; ISOTOPIC COMPOSITION; SEASONAL PATTERNS; SICHUAN BASIN; BROWN CARBON; RAINWATER;
D O I
10.1016/j.jes.2020.09.011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Precipitation represents an important phenomenon for carbon and nitrogen deposition. Here, the concentrations and fluxes of dissolved organic carbon (DOC) and total dissolved nitrogen (TDN) with their potential sources were analyzed in wet precipitation during summer monsoon from the Northern Indo-Gangetic Plain (IGP), important but neglected area. The volume-weighted mean (VWM) concentration of DOC and TDN were 687.04 and 1210.23 mu g/L, respectively. Similarly, the VWM concentration of major ions were in a sequence of NH4+ > Ca-2(+) > SO42- > Na+ > K+ > NO3- > Cl- > Mg2+ > F- > NO2-, suggesting NH4+ and Ca-2(+) from agricultural activities and crustal dust played a vital role in precipitation chemistry. Moreover, the wet deposition flux of DOC and TDN were 9.95 and 17.06 kg/(ha.year), respectively. The wet deposition flux of inorganic nitrogen species such as NH4+-N and NO3-N were 14.31 and 0.47 kg/(ha.year), respectively, demonstrating the strong influence of emission sources and precipitation volume. Source attribution from different analysis suggested the influence of biomass burning on DOC and anthropogenic activities (agriculture, animal husbandry) on nitrogenous species. The air-mass back trajectory analysis indicated the in- fluence of air masses originating from the Bay of Bengal, which possibly carried marine and anthropogenic pollutants along with the biomass burning emissions to the sampling site. This study bridges the data gap in the less studied part of the northern IGP region and provides new information for policy makers to deal with pollution control. (C) 2020 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:37 / 52
页数:16
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