Numerical study on the extinction dynamics of partially premixed meso-scale methane-air jet flames with hydrogen addition

In this paper, a model of partially premixed jet flames that sustained above a meso-scale short tube was established for an individual flame port of domestic gas stoves. The effects of hydrogen addition (volume ratio beta = 0%, 10%, 20%, 30%) on the extinction dynamics of CH4-air jet flames were numerically investigated. It is found that flame oscillation occurs once (beta = 10% and 20%) or twice (beta = 30%) in the extinction process. Moreover, the larger of beta, the longer the extinction process can sustain. Analysis was performed in terms of both chemical effect and thermal effect. As to the chemical effect, in the first place, the reaction rate decreases as the inlet velocity is reduced. As a result, the consumption rate of O-2 will be less than the supply rate from the incoming mixture, which makes the O-2 concentration in the flame center increase. On the other hand, the amount of H radicals increases with the increase of beta, and when the O-2 content at the flame center reaches a "critical point", the key elementary reaction "H + O-2 <-> O + OH " will be enhanced and consequently the total reaction rate will also be intensified. After that, the consumption rate of O-2 will be larger than the supply rate due to the reduced flow rate of incoming mixture. The total heat release rate will decrease sharply and extinction occurs. As regards the thermal effect, it is revealed that heat recirculation effect (indirect preheating effect) lags behind the variation of the reaction zone (i.e., flame), thus, it has a negligible impact on flame oscillation. In contrast, the preheating temperature in the vicinity of flame front (named as "direct pre-heating effect") exhibits a similar variation tendency with the total heat release rate of the flame. And the larger of beta, the more remarkable of the direct preheating effect can be. In summary, due to the chemical effect and thermal effect caused by hydrogen addition, the flame can survive for a longer time with fluctuation during the extinction process. (c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.