Direct Enhancement of Nuclear Singlet Order by Dynamic Nuclear Polarization

被引:86
|
作者
Tayler, Michael C. D. [1 ]
Marco-Rius, Irene [2 ,3 ]
Kettunen, Mikko I. [2 ,3 ]
Brindle, Kevin M. [2 ,3 ]
Levitt, Malcolm H. [1 ]
Pileio, Giuseppe [1 ]
机构
[1] Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England
[2] Univ Cambridge, Dept Biochem, Cambridge CB2 1GA, England
[3] Canc Res UK Cambridge Res Inst, Cambridge CB2 0RE, England
基金
英国工程与自然科学研究理事会; 欧洲研究理事会;
关键词
PARA-HYDROGEN; STATE;
D O I
10.1021/ja302814e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Hyperpolarized singlet order is available immediately after dissolution DNP, avoiding need for additional preparation steps. We demonstrate this procedure on a sample of [1,2-C-13(2)]pyruvic acid.
引用
收藏
页码:7668 / 7671
页数:4
相关论文
共 50 条
  • [1] Photochemically Induced Dynamic Nuclear Polarization of Heteronuclear Singlet Order
    Sheberstov, Kirill F.
    Chuchkova, Liubov
    Hu, Yinan
    Zhukov, Ivan, V
    Kiryutin, Alexey S.
    Eshtukov, Artur, V
    Cheshkov, Dmitry A.
    Barskiy, Danila A.
    Blanchard, John W.
    Budker, Dmitry
    Ivanov, Konstantin L.
    Yurkovskaya, Alexandra, V
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2021, 12 (19): : 4686 - 4691
  • [2] Singlet fission as a polarized spin generator for dynamic nuclear polarization
    Kawashima, Yusuke
    Hamachi, Tomoyuki
    Yamauchi, Akio
    Nishimura, Koki
    Nakashima, Yuma
    Fujiwara, Saiya
    Kimizuka, Nobuo
    Ryu, Tomohiro
    Tamura, Tetsu
    Saigo, Masaki
    Onda, Ken
    Sato, Shunsuke
    Kobori, Yasuhiro
    Tateishi, Kenichiro
    Uesaka, Tomohiro
    Watanabe, Go
    Miyata, Kiyoshi
    Yanai, Nobuhiro
    NATURE COMMUNICATIONS, 2023, 14 (01)
  • [3] Singlet fission as a polarized spin generator for dynamic nuclear polarization
    Yusuke Kawashima
    Tomoyuki Hamachi
    Akio Yamauchi
    Koki Nishimura
    Yuma Nakashima
    Saiya Fujiwara
    Nobuo Kimizuka
    Tomohiro Ryu
    Tetsu Tamura
    Masaki Saigo
    Ken Onda
    Shunsuke Sato
    Yasuhiro Kobori
    Kenichiro Tateishi
    Tomohiro Uesaka
    Go Watanabe
    Kiyoshi Miyata
    Nobuhiro Yanai
    Nature Communications, 14 (1)
  • [4] Dynamic Nuclear Polarization of 17O: Direct Polarization
    Michaelis, Vladimir K.
    Corzilius, Bjoern
    Smith, Albert A.
    Griffin, Robert G.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2013, 117 (48): : 14894 - 14906
  • [5] A Method for Dynamic Nuclear Polarization Enhancement of Membrane Proteins
    Smith, Adam N.
    Caporini, Marc A.
    Fanucci, Gail E.
    Long, Joanna R.
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2015, 54 (05) : 1542 - 1546
  • [6] POSITIVE ENHANCEMENT OF PROTON RESONANCES BY DYNAMIC NUCLEAR POLARIZATION
    DWEK, RA
    KENWORTHY, JG
    RICHARDS, RE
    MOLECULAR PHYSICS, 1966, 10 (06) : 529 - +
  • [7] Theoretical Aspects of the Cross Effect Enhancement of Nuclear Polarization under Static Dynamic Nuclear Polarization Conditions
    Kundu, Krishnendu
    Feintuch, Akiva
    Vega, Shimon
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2019, 10 (08): : 1769 - 1778
  • [8] Nuclear relaxation in dynamic nuclear polarization
    Popenko, N.A.
    Tarapov, S.I.
    Journal of Applied Spectroscopy, 1997, 64 (03): : 376 - 379
  • [9] Nuclear relaxation in dynamic nuclear polarization
    N. A. Popenko
    S. I. Tarapov
    Journal of Applied Spectroscopy, 1997, 64 (3) : 376 - 379
  • [10] Nuclear Relaxation in Dynamic Nuclear Polarization
    J Appl Spectrosc, 3 (376):