Arbitrary-detuning asynchronous optical sampling pump-probe spectroscopy of bacterial reaction centers

被引:15
|
作者
Antonucci, Laura [1 ,2 ]
Bonvalet, Adeline [1 ,2 ]
Solinas, Xavier [1 ,2 ]
Jones, Michael R. [3 ]
Vos, Marten H. [1 ,2 ]
Joffre, Manuel [1 ,2 ]
机构
[1] Ecole Polytech, CNRS, Lab Opt & Biosci, F-91128 Palaiseau, France
[2] INSERM, U696, F-91128 Palaiseau, France
[3] Univ Bristol, Sch Biochem, Bristol BS8 1TD, Avon, England
关键词
RHODOBACTER-SPHAEROIDES; PULSES; RATES;
D O I
10.1364/OL.38.003322
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A recently reported variant of asynchronous optical sampling compatible with arbitrary unstabilized laser repetition rates is applied to pump-probe spectroscopy. This makes possible the use of a 5.1 MHz chirped pulse oscillator as the pump laser, thus extending the available time window to almost 200 ns with a time resolution as good as about 320 fs. The method is illustrated with the measurement in a single experiment of the complete charge transfer dynamics of the reaction center from Rhodobacter sphaeroides. (C) 2013 Optical Society of America
引用
收藏
页码:3322 / 3324
页数:3
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