Validation of ozone measurements from the Atmospheric Chemistry Experiment (ACE)

被引：85

作者：

Dupuy, E. ^{[1
]}

Walker, K. A. ^{[1
,2
]}

Kar, J. ^{[2
]}

Boone, C. D. ^{[1
]}

McElroy, C. T. ^{[2
,3
]}

Bernath, P. F. ^{[1
,4
]}

Drummond, J. R. ^{[2
,5
]}

Skelton, R. ^{[1
]}

McLeod, S. D. ^{[1
]}

Hughes, R. C. ^{[1
]}

Nowlan, C. R. ^{[2
]}

Dufour, D. G. ^{[6
]}

Zou, J. ^{[2
]}

Nichitiu, F. ^{[2
]}

Strong, K. ^{[2
]}

Baron, P. ^{[7
]}

Bevilacqua, R. M. ^{[8
]}

Blumenstock, T. ^{[9
,10
]}

Bodeker, G. E. ^{[11
]}

Borsdorff, T. ^{[12
]}

Bourassa, A. E. ^{[13
]}

Bovensmann, H. ^{[14
]}

Boyd, I. S. ^{[15
]}

Bracher, A. ^{[14
]}

Brogniez, C. ^{[16
]}

Burrows, J. P. ^{[14
]}

Catoire, V. ^{[17
]}

Ceccherini, S. ^{[18
]}

Chabrillat, S. ^{[19
]}

Christensen, T. ^{[20
]}

Coffey, M. T. ^{[21
]}

Cortesi, U. ^{[18
]}

Davies, J. ^{[3
]}

De Clercq, C. ^{[19
]}

Degenstein, D. A. ^{[13
]}

Maziere, M. De ^{[19
]}

Demoulin, P. ^{[22
]}

Dodion, J. ^{[19
]}

Firanski, B. ^{[23
]}

Fischer, H. ^{[9
,10
]}

Forbes, G. ^{[24
]}

Froidevaux, L. ^{[25
]}

Fussen, D. ^{[19
]}

Gerard, P. ^{[19
]}

Godin-Beekmann, S. ^{[26
]}

Goutail, F. ^{[27
]}

Granville, J. ^{[19
]}

Griffith, D. ^{[28
]}

Haley, C. S. ^{[29
]}

Hannigan, J. W. ^{[21
]}

机构：

[1] Univ Waterloo, Dept Chem, Waterloo, ON N2L 3G1, Canada

[2] Univ Toronto, Dept Phys, Toronto, ON, Canada

[3] Environm Canada, Downsview, ON, Canada

[4] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England

[5] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS, Canada

[6] Picomole Instruments Inc, Edmonton, AB, Canada

[7] Natl Inst Informat & Commun Technol NICT, Koganei, Tokyo, Japan

[8] USN, Res Lab, Washington, DC 20375 USA

[9] Forschungszentrum Karlsruhe, Inst Meteorol & Klimaforsch, D-76021 Karlsruhe, Germany

[10] Univ Karlsruhe, Karlsruhe, Germany

[11] Natl Inst Water & Atmospher Res, Lauder, New Zealand

[12] Forschungszentrum Karlsruhe, Inst Meteorol & Klimaforsch Atmosphar Umweltforsc, Garmisch Partenkirchen, Germany

[13] Univ Saskatchewan, Inst Space & Atmospher Studies, Saskatoon, SK S7N 0W0, Canada

[14] Univ Bremen, IUP, Bremen, Germany

[15] Univ Massachusetts, NIWA Environm Res Inst, Amherst, MA 01003 USA

[16] Univ Lille 1, Opt Atmospher Lab, CNRS, F-59655 Villeneuve Dascq, France

[17] Univ Orleans, CNRS, Lab Phys & Chim Environm, Orleans, France

[18] CNR, Inst Fis Applicata N Carrara IFAC, Sesto Fiorentino, Italy

[19] Inst Aeron Spatiale Belgique BIRA IASB, Brussels, Belgium

[20] Danish Meteorol Inst, Danish Climate Ctr, Copenhagen, Denmark

[21] Natl Ctr Atmospher Res, Earth & Sun Syst Lab, Boulder, CO 80307 USA

[22] Univ Liege, Inst Astrophys & Geophys, Liege, Belgium

[23] Environm Canada, Ctr Atmospher Res Expt, Sci & Technol Branch, Egbert, ON, Canada

[24] Environm Canada Sable Isl, Dartmouth, NS, Canada

[25] CALTECH, Jet Prop Lab, Pasadena, CA USA

[26] Univ Paris 06, CNRS, Serv Aeron, Paris, France

[27] CNRS, Serv Aeron, F-91371 Verrieres Le Buisson, France

[28] Univ Wollongong, Sch Chem, Wollongong, NSW, Australia

[29] York Univ, Ctr Res Earth & Space Sci, Toronto, ON M3J 2R7, Canada

[30] York Univ, Dept Earth & Space Sci & Engn, Toronto, ON M3J 2R7, Canada

[31] Chalmers Univ Technol, Dept Radio & Space Sci, S-41296 Gothenburg, Sweden

[32] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA

[33] Fujitsu FIP Corp, Tokyo, Japan

[34] Australian Antarctic Div, Ice Ocean Atmosphere & Climate IOAC Program, Kingston, Australia

[35] Finnish Meteorol Inst, Earth Observat, FIN-00101 Helsinki, Finland

[36] New Mexico Inst Min & Technol, Socorro, NM 87801 USA

[37] GATS Inc, Newport News, VA USA

[38] NASA, Langley Res Ctr, Div Atmospher Sci, Hampton, VA 23665 USA

[39] Table Mt Facil, Jet Prop Lab, Wrightwood, CA USA

[40] Univ Massachusetts, Dept Astron, Amherst, MA 01003 USA

[41] La Trobe Univ, Dept Phys, Bundoora, Vic 3086, Australia

[42] Univ Oxford, Oxford OX1 2JD, England

[43] Univ Colorado, Atmospher & Space Phys Lab, Boulder, CO 80309 USA

[44] Natl Inst Publ Hlth & Environm RIVM, Bilthoven, Netherlands

[45] Penn State Univ, Dept Meteorol, University Pk, PA 16802 USA

[46] Bur Meteorol, Atmosphere Watch Sect, Melbourne, Vic, Australia

[47] Alfred Wegener Inst Polar & Marine Res, Res Unit Potsdam, Potsdam, Germany

[48] Sci Syst & Applicat Inc, Lanham, MD USA

[49] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA

来源：

ATMOSPHERIC CHEMISTRY AND PHYSICS | 2009年 / 9卷 / 02期

基金：

加拿大自然科学与工程研究理事会;

关键词：

GROUND-BASED FTIR; LIMB SCATTER MEASUREMENTS; TECHNICAL NOTE; STRATOSPHERIC OZONE; POAM-III; SAGE-II; VERTICAL-DISTRIBUTION; ERROR ANALYSIS; O-3; PROFILES; GEOPHYSICAL VALIDATION;

D O I：

10.5194/acp-9-287-2009

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

This paper presents extensive bias determination analyses of ozone observations from the Atmospheric Chemistry Experiment (ACE) satellite instruments: the ACE Fourier Transform Spectrometer (ACE-FTS) and the Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (ACE-MAESTRO) instrument. Here we compare the latest ozone data products from ACE-FTS and ACE-MAESTRO with coincident observations from nearly 20 satellite-borne, airborne, balloon-borne and ground-based instruments, by analysing volume mixing ratio profiles and partial column densities. The ACE-FTS version 2.2 Ozone Update product reports more ozone than most correlative measurements from the upper troposphere to the lower mesosphere. At altitude levels from 16 to 44 km, the average values of the mean relative differences are nearly all within +1 to +8%. At higher altitudes (45 60 km), the ACE-FTS ozone amounts are significantly larger than those of the comparison instruments, with mean relative differences of up to +40% (about + 20% on average). For the ACE-MAESTRO version 1.2 ozone data product, mean relative differences are within +/- 10% (average values within +/- 6%) between 18 and 40 km for both the sunrise and sunset measurements. At higher altitudes (similar to 35-55 km), systematic biases of opposite sign are found between the ACE-MAESTRO sunrise and sunset observations. While ozone amounts derived from the ACE-MAESTRO sunrise occultation data are often smaller than the coincident observations (with mean relative differences down to -10%), the sunset occultation profiles for ACE-MAESTRO show results that are qualitatively similar to ACE-FTS, indicating a large positive bias (mean relative differences within +10 to +30%) in the 45-55 km altitude range. In contrast, there is no significant systematic difference in bias found for the ACE-FTS sunrise and sunset measurements.

引用

页码：287 / 343

页数：57

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